Magnetism and electronic order in SmTiO$_{\mathrm{3}}$ quantum well heterostructures

ORAL

Abstract

Complex oxide heterostructures that possess high density interfacial electron gases due to charge discontinuities between neighboring layers provide a unique platform with which to study correlated electron physics. In heterostructures containing band insulator SrTiO$_{\mathrm{3}}$ and Mott insulating rare earth titanate layers, it has been shown that tuning relative layer thicknesses can in turn tune both the electronic and magnetic properties found in each layer type, leading to exotic metal-insulator transitions and electronic symmetry breaking in the interleaving quantum wells. Here we use a combination of resonant x-ray reflectometry (RXR), polarized neutron reflectometry (PNR), and muon spin rotation (muSR) to probe the electronic and magnetic properties of SmTiO$_{\mathrm{3}}$ thin films and SrTiO$_{\mathrm{3}}$-SmTiO$_{\mathrm{3}}$ heterostructures. RXR measurements demonstrate the effect of tuning both SrTiO$_{\mathrm{3}}$ and SmTiO$_{\mathrm{3}}$ layer thicknesses on the electronic structure, and our combined PNR and muSR results resolve the freezing of interface-induced free electrons within the SrTiO$_{\mathrm{3}}$ quantum wells below a critical temperature. The correlations between our scattering results and previously reported anomalous transport in SrTiO$_{\mathrm{3}}$-SmTiO$_{\mathrm{3}}$ heterostructures will be discussed.

Authors

  • Ryan Need

    • Materials Department, University of California Santa Barbara
  • Patrick Marshall

    • Materials Department, University of California Santa Barbara
  • Brandon Isaac

    • Materials Department, University of California Santa Barbara
  • Eugen Weschke

    • BESSY-II, Helmholtz Zentrum Berlin
  • Andreas Suter

    • Swiss Muon Source, Paul Scherrer Institute
  • Michael Graf

    • Physics Department, Boston College
  • Susanne Stemmer

    • Materials Department, University of California Santa Barbara
  • Stephen Wilson

    • Materials Department, University of California Santa Barbara