Pb temperature determination using L-edge Extended X-ray Absorption Fine Structure

ORAL

Abstract

The temperature of dynamically compressed materials is the largest uncertainty in modern equation of state modeling, and developing new tools to measure temperature is important to complement data from existing diffraction and equation-of-state platforms. In experiments performed at the National Ignition Facility (NIF), we measured L-edge extended x-ray absorption fine structure (EXAFS) of dynamically-compressed Pb up to 300 GPa. These modulations in the x-ray absorption are caused by photoelectron scattering off nearby atoms, and are sensitive to both local atomic spacing and thermal disorder. The measured EXAFS are interpreted using density functional theory (DFT) and molecular dynamics (MD) simulations and compared agonist temperature determined using diffraction data in a different platform.

*This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

Publication: H. Sio, et al., Rev. Sci. Instrum. 95, 103523 (2024)

Presenters

  • Hong W Sio

    • Lawrence Livermore National Laboratory

Authors

  • Hong W Sio

    • Lawrence Livermore National Laboratory
  • Andrew Krygier

    • Lawrence Livermore National Laboratory
  • Stanimir A Bonev

    • Lawrence Livermore National Laboratory
    • Lawrence Livermore Natl Lab
  • Amy L Coleman

    • Lawrence Livermore National Laboratory
  • Robert E Rudd

    • Lawrence Livermore National Laboratory
  • Stanislav Stoupin

    • Lawrence Livermore National Laboratory
  • Bernard Kozioziemski

    • Lawrence Livermore National Laboratory
  • James M McNaney

    • Lawrence Livermore National Laboratory
  • Jon H Eggert

    • Lawrence Livermore National Laboratory
  • Yuan Ping

    • Lawrence Livermore National Laboratory