Direct observation of an abrupt insulator-to-metal transition in dense liquid deuterium

ORAL

Abstract

Recently a so-called shock-ramp platform has been developed on the Sandia Z Accelerator to access off-Hugoniot states in liquids. The accelerator delivers a two-step current pulse; the first accelerates the electrode to a reasonably constant velocity, which upon impact with the sample cell creates a well-defined shock, the subsequent current rise produces ramp compression from the initially shocked state. This technique generates relatively cool ($\sim$1-2 kK), high pressure ($>$300 GPa), high compression ($\sim$10-15 fold compression) states, allowing experimental access to the region of phase space where hydrogen is predicted to undergo a first-order phase transition from an insulating molecular-like liquid to a conducting atomic-like liquid. In this talk we will discuss the experimental platform, survey the various theoretical predictions for the liquid-liquid, insulator-to-metal transition in hydrogen, and present the results of experiments that clearly show an abrupt transition to a metallic state. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000.

Authors

  • Marcus Knudson

    • Sandia National Laboratories Albuquerque
    • Sandia National Laboratories
  • Michael Desjarlais

    • Sandia National Laboratories
  • Andeas Becker

    • University of Rostock
  • Raymond Lemke

    • Sandia National Laboratories
  • Kyle Cochrane

    • Sandia National Laboratories
  • Mark Savage

    • Sandia National Laboratories
  • David Bliss

    • Sandia National Laboratories
  • Thomas Mattsson

    • Sandia National Laboratories
  • Ronald Redmer

    • University of Rostock