Ammonia ice at very high pressure

ORAL

Abstract

In this presentation, we report an extended experimental investigation of the phase diagram of ammonia at high pressure and temperature. By combining Raman scattering and X-ray diffraction experiments, we demonstrate the presence of a new H-disordered crystalline form above $\sim$60 GPa and $\sim$700 K. Using \textit{ab initio} MD simulations, we show that this new disordered phase is a superionic conductor. We will also present new experimental results (infrared, Raman and X-ray) on NH$_{3}$ and ND$_{3}$ at ambient temperature up to 200 GPa and will discuss the existence of ionic ammonia ices.

Authors

  • Sandra Ninet

    • Universite Pierre et Marie Curie - Institut de Mineralogie et de Physique des Milieux Condens\'es - Paris VI, France
  • Frederic Datchi

    • Universite Pierre et Marie Curie - Institut de Mineralogie et de Physique des Milieux Condenses - Paris VI, France
  • Paul Dumas

    • Synchrotron SOLEIL, Gif Sur Yvette, France
    • Synchrotron SOLEIL, Gif-sur-Yvette, France
  • Mohamed Mezouar

    • European Synchrotron Radiation Facility, Grenoble, France
    • European Synchrotron Radiation Facility (ESRF); Grenoble; France
    • ESRF
  • Gaston Garbarino

    • European Synchrotron Radiation Facility, Grenoble, France
    • European Synchrotron Radiation Facility (ESRF); Grenoble; France
    • ESRF
  • Adrien Mafety

    • Universite Pierre et Marie Curie - Institut de Mineralogie et de Physique des Milieux Condenses - Paris VI, France
  • Chris Pickard

    • Department of Physics and Astronomy, University College London, United Kingdom
  • Richard Needs

    • Theory of Condensed Matter Group, Cavendish Laboratory, Cambridge, United Kingdom
    • University of Cambridge
  • Marco Saitta

    • Universit\'e Pierre et Marie Curie - Institut de Min\'eralogie et de Physique des Milieux Condens\'es - Paris VI, France