Flow Properties of a Twist-bend Nematic Liquid Crystal

ORAL

Abstract

We present the first shear alignment studies and rheological measurements in the twist-bend nematic ($N_{tb} )$ liquid crystal phase of odd numbered flexible dimer molecules. It is found that the $N_{tb} $ phase is strongly shear-thinning. At shear stresses below $1Pa$ the apparent viscosity of $N_{tb} $ is $1000$ times larger than in the nematic phase. At stress above $10Pa$ the $N_{tb} $ viscosity drops by two orders of magnitude and the material exhibits Newtonian fluid behavior. This is consistent with the heliconic axis becoming normal to the shear plane via shear-induced alignment. From measurements of the dynamic modulus we estimate the compression modulus of the pseudo-layers to be $B\sim 2kPa$; this value is discussed within the context of a simple theoretical model based upon a coarse-grained elastic free energy.

Authors

  • Seyyed Muhammad Salili

    • Chemical Physics Interdisciplinary Program and Liquid Crystal Institute, Kent State University, Kent, OH 44242
  • Chanjoong Kim

    • Liquid Crystal Institute, Kent State University, Kent, OH 44242
    • Chemical Physics Interdisciplinary Program and Liquid Crystal Institute, Kent State University, Kent, OH 44242
  • Samuel Sprunt

    • Department of Physics, Kent State University, Kent, OH 44242
    • Department of Physics, Kent State Univ - Kent
  • James Gleeson

    • Kent State University
    • Department of Physics, Kent State University, Kent, OH 44242
    • Department of Physics, Kent State Univ - Kent
  • Owain Parri

    • Merck Chemicals Ltd., Chilworth Technical Centre, University Parkway, Southampton SO16 7QD, UK
  • Antal Jakli

    • Kent State University
    • Chemical Physics Interdisciplinary Program and Liquid Crystal Institute, Kent State University, Kent, OH 44242
    • Liquid Crystal Institute, Kent State Univ - Kent