Quantum-critical scaling in the Mn-based kagome metal Sc<sub>3</sub>Mn<sub>3</sub>Al<sub>7</sub>Si<sub>5</sub>

ORAL

Abstract

Kagome lattices can host a variety of exotic ground states, including quantum spin liquids and correlated phases associated with dispersionless flat energy bands. The Mn-based kagome metal Sc3Mn3Al7Si5 crystalizes a hexagonal structure in which Mn ions form a kagome network, and shows unusual behavior in transport and thermodynamic properties [1]. Interestingly, a recent study, supported by theoretical calculations, has suggested the presence of orbital-selective flat-band-induced ferromagnetic fluctuations [2]. To elucidate the flat-band-induced ferromagnetic instability, we synthesized single crystals of Sc3Mn3Al7Si5 and measured charge transport and heat capacity at very low temperatures. We observe no anomaly associated with long-range order in resistivity down to 15 mK and a logarithmic divergence in low-temperature heat capacity. The logarithmic divergence in heat capacity is strongly suppressed by magnetic fields, suggesting a crossover from non-Fermi-liquid to Fermi-liquid behavior, often observed in quantum critical metals. This anomalous crossover in heat capacity is well described by quantum-critical scaling. We will discuss the relationship between the quantum criticality and orbital-selective flat bands in the kagome metal Sc3Mn3Al7Si5.

*C.D. and Y.N. were supported by an NSF Career DMR-1944975. The National High Magnetic Field Laboratory is supported by the National Science Foundation through NSF/DMR-1644779 and the State of Florida.

Publication: [1] H. He et al., Inorganic Chemistry 53, 17 (2014).
[2] S. Samanta et al., arXiv:2304.04928.

Presenters

  • Yasuyuki Nakajima

    • University of Central Florida

Authors

  • Yasuyuki Nakajima

    • University of Central Florida
  • Charuni Dissanayake

    • University of Central Florida
  • Kapila Kumarasinghe

    • University of Central Florida
  • Mark Tomlinson

    • University of Central Florida
  • Eun Sang Choi

    • National High Magnetic Field Laboratory
    • National High Magnetic Field Lab, Tallahassee, Florida
    • NHMFL
    • MagLab
    • Florida State University
    • National High Magnetic Field Laboratory, Florida State University