New Color Centers in Diamond for Quantum Applications

ORAL

Abstract

Color centers in diamond are promising platforms for quantum communication and quantum sensing applications. All the defects in diamond reported so far emit photons in the visible to near-infrared region, which experience high losses in fiber optics and scattering media such as biological samples. Furthermore, no color centers observed thus far exhibit coherence times comparable to nitrogen vacancies at elevated temperatures. Here, we report the experimental observation of two new color centers in diamond that emit in the telecom band. The first color center emits in the telecom O-band [1]. From absorption, photoluminescence, and transient absorption spectroscopy, we identify a zero-phonon line at 1221 nm with phonon replicas separated by 42 meV and an excited state lifetime of ~270 ps. The second is substitutional Er3+ incorporated in diamond, which emits in the telecom C-band. Finally, we deploy our spectroscopy and materials characterization pipeline to investigate other new defects in diamond as potential candidates for quantum sensing by characterizing spin dynamics using pulsed electron spin resonance.



[1] S. Mukherjee et al., Nano Lett. 2023, 23, 7, 2557–2562.

Publication: S. Mukherjee et al., Nano Lett. 2023, 23, 7, 2557–2562.

Presenters

  • Sounak Mukherjee

    • Princeton University

Authors

  • Sounak Mukherjee

    • Princeton University
  • Zihuai Zhang

    • University of California, Berkeley and Lawrence Berkeley National Laboratory
    • Princeton University
    • University of California, Berkeley
    • University of California, Berkeley; Lawrence Berkeley National Laboratory
  • Sean Karg

    • Princeton University
  • Arunava Das

    • Princeton University
  • Daniel G Oblinsky

    • Princeton University
  • Sebastian P Horvath

    • Princeton University
  • Mayer M Feldman

    • Princeton University
  • Mitchell O de Vries

    • RMIT University
  • Brett C Johnson

    • RMIT University
  • Brant C Gibson

    • RMIT University
  • Edwin L H Mayes

    • RMIT University
  • Andrew M Edmonds

    • Element Six
  • Nicola Palmer

    • Element Six
  • Matthew L Markham

    • Element Six
  • Ádám Gali

    • Wigner Research Centre for Physics
  • Gergő Thiering

    • Wigner Research Centre for Physics
    • Wigner Research Centre
  • Adam Dalis

    • Hyperion Materials & Technologies
  • Timothy Dumm

    • Hyperion Materials & Technologies
  • Gregory D Scholes

    • Princeton University
  • Alastair Stacey

    • RMIT University
    • School of Science, RMIT University, Melbourne, Victoria 3000, Australia
  • Philipp Reineck

    • RMIT University
  • Jeff D Thompson

    • Princeton University
  • Stephen A Lyon

    • Princeton, EeroQ Corp.
    • Princeton University, EeroQ Corp
    • Princeton University, EeroQ Corp.
    • Princeton University
  • Nathalie P de Leon

    • Princeton University