Two-Fold Anisotropic Superconductivity in Bilayer T<sub>d</sub>-MoTe<sub>2</sub>

ORAL

Abstract

Non-centrosymmetric 2D superconductors offer an opportunity to explore superconducting behaviors with strong spin-orbit coupling. Among the non-centrosymmetric families, Td-MoTe2 is a representative material because of its rich phases. Notably, Td-MoTe2 is the first 2D materials that demonstrated a coupling between ferroelectricity and superconductivity, and this ferroelctric switching can be simply controlled by electrical gating. Here, we will present on the superconducting behavior in bilayer Td-MoTe2 under an applied magentic field along different directions in-plane, and under different displacement fields and doping densities. We find that bilayer Td-MoTe2 has a two-fold symmetric superconducting behavior as a function of in-plane magnetic field angle that maximizes along the a-axis, parallel to the mirror plane. Importantly, large violations of Pauli limiting are observed, and DFT calculation suggests the anisotropic superconductivity in bilayer MoTe2 is likely driven by Ising-like spin-orbit coupling. In addition, the two-fold anisotropy is preserved in the entire superconducting region, even with the interaction of strong Rashba spin-orbit coupling, and we find that the two-fold symmetric superconductivity remains after the ferroelectric switching. Our findings generally agree with previously observed results in multilayer and monolayer Td-MoTe2 and the expected spin-orbit enhanced upper critical fields as found in DFT calculations.

*We would like to acknowledge support from the Department of Energy BES program (DE-SC0023866).

Presenters

  • Zizhong Li

    • University of Wisconsin - Madison

Authors

  • Zizhong Li

    • University of Wisconsin - Madison
  • Apoorv Jindal

    • Columbia University
  • Alex Strasser

    • Texas A&M University
  • Yangchen He

    • University of Wisconsin Madison
    • University of Wisconsin - Madison
  • David E Graf

    • Florida State University
    • National High Magnetic Fields Laboratory, Florida State University
    • National High Magnetic Field Laboratory, Florida State University
  • Wenkai Zheng

    • National High Magnetic Field Laboratory
  • Kenji Watanabe

    • National Institute for Materials Science
    • NIMS
    • Research Center for Electronic and Optical Materials, National Institute for Materials Science
    • Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science
  • Takashi Taniguchi

    • Kyoto Univ
    • National Institute for Materials Science
    • Research Center for Materials Nanoarchitectonics
    • Research Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • National Institute for Materials Sciences
    • NIMS
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science
    • International Center for Materials Nanoarchitectonics, NIMS, Japan
    • International Center for Materials Nanoarchitectonics, Tsukuba
    • National Institue for Materials Science
    • Kyoto University
    • National Institute of Materials Science
    • International Center for Materials Nanoarchitectonics and National Institute for Materials Science
  • Luis Balicas

    • National High Magnetic Field Laboratory
    • Florida State University, National High Magnetic Field Laboratory
  • Xiaofeng Qian

    • Texas A&M University
  • Abhay N Pasupathy

    • Columbia University
    • Columbia University & Brookhaven National Laboratory
  • Daniel Rhodes

    • University of Wisconsin - Madison