Near-field THz spectroscopy of tantalum films for superconducting quantum devices

ORAL

Abstract

Superconducting quantum circuits are one of the leading quantum computing platforms. To advance superconducting quantum computing to a point of practical importance, it is critical to identify and address material imperfections that lead to decoherence. In this talk, I will show how terahertz Scanning Near-field Optical Microscopy (SNOM) can be used to probe functional devices such as coplanar microwave resonators and inform the processing of new materials for quantum technology. I will discuss the recent observation of a localized vibrational excess on the surface of tantalum films and how this excess is connected to the boson peak, a universal signature of amorphous materials. The nanoscale identification and localization of amorphous oxides provides critical insight as amorphous materials host tunneling two level systems (TLS) – the major performance limiting factor in superconducting quantum devices.

*Financial support provided by the Australian Research Council DP210103342, CE170100009, the Foundational Questions Institute Fund (Grant FQXi-IAF19-04), and Research Foundation - Flanders (FWO, Grants 12Y7221N and V400622N).

Publication: X. Guo, Z. Degnan, J.A. Steele, E. Solano, B.C. Donose, K. Bertling, A. Fedorov, A.D. Rakić, P. Jacobson J. Phys. Chem. Lett. 14, 4892 (2023)
X. Guo, X. He, Z. Degnan, B.C. Donose, K. Bertling, A. Fedorov, A.D. Rakić, P. Jacobson Appl. Phys. Lett. 119, 091101 (2021)
X. Guo, X. He, Z. Degnan, C.-C. Chiu, B.C. Donose, K. Bertling, A. Fedorov, A.D. Rakić, P. Jacobson Nanophotonics 12, 1865 (2023)

Presenters

  • Peter A Jacobson

    • University of Queensland

Authors

  • Peter A Jacobson

    • University of Queensland
  • Xiao Guo

    • University of Queensland
  • Zachary Degnan

    • University of Queensland
  • Julian Steele

    • University of Queensland
  • Eduardo Solano

    • ALBA Synchrotron Light Source
  • Bogdan C Donose

    • University of Queensland
  • Karl Bertling

    • University of Queensland
  • Arkady Fedorov

    • University of Queensland
  • Aleksandar D Rakić

    • University of Queensland