Low-energy charge dynamics of infinite-layer nickelates: evidence for d-wave superconductivity

ORAL

Abstract

The discovery of superconductivity in infinite-layer nickelates establishes a new category of unconventional superconductors that shares structural and electronic similarities with cuprates. Despite the exciting advances, the key issues of the superconducting pairing symmetry, gap amplitude, superconducting fluctuation and collective modes remain elusive. In this talk, I will show how we utilize static and ultrafast terahertz spectroscopy to address these outstanding problems. We demonstrate that the equilibrium terahertz conductivity and nonequilibrium terahertz responses of an optimally Sr-doped nickelate film (Tc = 17 K) are in line with the electrodynamics of d-wave superconductivity in the dirty limit. The gap-to-Tc ratio is extracted to be 3.4, which indicates the superconductivity falls in the weak-coupling regime. In addition, we observed significant superconducting fluctuation near Tc. These results highlights a new d-wave system which closely resembles the electron-doped cuprates, expanding the family of unconventional superconductivity in oxides. Finally, we will present evidence for highly damped Higgs mode in infinite-layer nickelates.

*This work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering (Ames National Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358). Work at SIMES was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division under Contract No. DE-AC02-76SF00515 and the Gordon and Betty Moore Foundation’s Emergent Phenomena in Quantum Systems Initiative.

Publication: arXiv:2310.02586 (2023)
arXiv:2310.02589 (2023)

Presenters

  • Bing Cheng

    • Ames National Laboratory

Authors

  • Bing Cheng

    • Ames National Laboratory
  • Di Cheng

    • Iowa State University
  • Kyuho Lee

    • Stanford University
  • Liang Luo

    • Ames National Laboratory
    • Ames Laboratory
  • Zhuoyu Chen

    • Stanford University
  • Yonghun Lee

    • Stanford University
  • Bai Yang Wang

    • Stanford University
  • Martin Mootz

    • Iowa State University
    • Ames National Laboratory
  • Chuankun Huang

    • Iowa State University
  • Ilias Perakis

    • University of Alabama at Birmingham
  • Zhi-Xun Shen

    • Stanford University
    • stanford university
  • Harold Hwang

    • Stanford University
  • JIGANG Wang

    • Iowa State University