micro-ARPES imaging of the conduction band and moiré replicas in 2D semiconductors

ORAL

Abstract

We present measurements of the conduction band in WS2-on-WSe2 moiré heterobilayers using submicron angle-resolved photoemission spectroscopy The heterobilayers are partially capped by graphene and are electrostatically doped in situ. We find that, at all twist angles, the conduction band edge is the WS2 K-point valley while the Q-point valley is at slightly higher energy. The measured band gap is 1.58 ± 0.03 eV and in one device we observe the conduction band curvature with an effective mass of 0.15me. We also observe replicas of the WS2 conduction band displaced by reciprocal lattice vectors of the moiré superlattice, whose three-fold intensity pattern can be explained by interference between multiple moiré potential-induced scattering pathways.

*U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under award DE-SC0019443.

Publication: "Imaging the conduction band and moiré replicas in 2D semiconductors", Abigail J Graham, Heonjoon Park, Paul V. Nguyen, James Nunn, Viktor Kandyba, Mattia Cattelan, Alessio Giampietri, Alexei Barinov, David H. Cobden, Xiaodong Xu, Neil R. Wilson (in prep.)

Presenters

  • Paul V Nguyen

    • University of Washington

Authors

  • Paul V Nguyen

    • University of Washington
  • Abigail J Graham

    • University of Warwick
  • Heonjoon Park

    • University of Washington
  • James Nunn

    • University of Warwick
  • Viktor Kandyba

    • Elettra - Sincrotrone Trieste S.C.p.A.
  • Mattia Cattelan

    • Elettra - Sincrotrone Trieste S.C.p.A.
  • Alessio Giampietri

    • Elettra - Sincrotrone Trieste S.C.p.A.
  • Alexei V Barinov

    • Elettra - Sincrotrone Trieste S.C.p.A.
  • Anton Andreev

    • University of Washington
  • Mark Rudner

    • University of Washington
  • Xiaodong Xu

    • University of Washington
  • Neil R Wilson

    • University of Warwick
  • David H Cobden

    • University of Washington