Wide Field Imaging of Low-dimensional Magnetism by 2D Spin Defects

ORAL

Abstract

Quantum sensing using atomic spin defects serves as a transformative method to explore the local magnetic properties of solid-state systems with optimal spatial and field sensitivity. The flourishing catalog of van der Waals two-dimensional (2D) materials has provided a diverse new playground to enrich this field. In comparison with their conventional counterparts imbedded in three-dimensional solid-state-media, spin defects hosted by 2D materials exhibit improved versatility and remarkable compatibility to device integration. In this work, we report nanoscale quantum sensing and imaging of exfoliated 2D ferromagnet Fe3GeTe2 flakes by boron vacancy spin defects in an adjacent hexagonal boron nitride capping layer. Exploiting the wide field magnetometry method, we directly imaged the local magnetic texture of the Fe3GeTe2 flake and its characteristic temperature and field dependent magnetization evolution behavior. We highlight that the presented quantum sensing platform can be extended naturally to a large family of miniaturized 2D van der Waals heterostructures, bringing ample opportunities to the forefront research of quantum material and quantum sensing.

*This work is supported by the Air Force Office of Scientific Research under award FA9550-20-1-0319 and its Young Investigator Program under award FA9550-21-1-0125, U. S. National Science Foundation (NSF) under award ECCS-2029558 and DMR-2046227. M. A. and J. S. were supported by NSF under the award ECCS-2051450.

Publication: M. Huang, J. Zhou, D. Chen, H. Lu, N. J. McLaughlin, S. Li, M. Alghamdi, D. Djugba, J. Shi, H. L. Wang, and C. H. R. Du, Wide Field Imaging of van der Waals Ferromagnet Fe3GeTe2 by Spin Defects in Hexagonal Boron Nitride, Nature Communications 13, 5369 (2022).

Presenters

  • Jingcheng Zhou

    • University of California, San Diego

Authors

  • Jingcheng Zhou

    • University of California, San Diego
  • Mengqi Huang

    • University of California, San Diego
  • Di Chen

    • University of Houston
  • Hanyi Lu

    • University of California San Diego
    • University of California, San Diego
  • Nathan J McLaughlin

    • University of California, San Diego
  • Senlei Li

    • University of California, San Diego
  • Mohammed A Alghamdi

    • University of California, Riverside
  • Dziga Djugba

    • University of California San Diego
    • University of California, San Diego
  • Jing Shi

    • University of California, Riverside
  • Hailong Wang

    • University of California, San Diego
  • Chunhui R Du

    • University of California, San Diego