Antiferromagnetism and field-induced transitions in single crystals of the Remeika phase compound Nd<sub>3</sub>Rh<sub>4</sub>Ge<sub>13</sub>
ORAL
Abstract
Remeika phases with the chemical formula R3T4M13 (R = rare earth, T = transition metal, M = group 14 metals) make up a vast family of intermetallic compounds. This caged structure of the Remeika phase results in a wide range of physical properties, including superconductivity, quantum criticality, and structural distortions, making their characteristics strikingly different for each material. In this talk, we report the first-ever single crystal growth and characterization of Nd3Rh4Ge13 utilizing susceptibility, heat capacity, and electrical transport measurements. Nd3Rh4Ge13 crystallizes in the Yb3Rh4Sn13 cubic structure type and orders antiferromagnetically below TN = 1.6K. In addition, we see evidence of meta-magnetic transitions emerging from the ordered state. We also explore the possibility of iso-valent substitution of rhodium, thereby tuning the spin-orbit coupling (SOC) strength and exchange interactions. These systems allow us to study how the SOC influences the magnetic structures and properties of the rare-earth-based Remeika phases.
*This work was supported by the Natural Sciences and Engineering Research Council of Canada. This research was undertaken thanks in part to funding from the Canada First Research Excellence Fund, Quantum Materials and Future Technologies Program.
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Presenters
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Samikshya Sahu
- The University of British Columbia