Scattering-Type Scanning Near-Field Optical Microscopy with Akiyama Piezo-Probes in High Magnetic Fields

ORAL

Abstract

Recent developments of the scattering-type scanning near-field optical microscope at cryogenic temperatures (cryo-SNOM) have led to many breakthroughs in the studies of low energy excitations in quantum materials. However, the simultaneous demands on vibration isolation, low base temperature, precise nano-positioning, and optical access make the construction of a cryo-SNOM a daunting task. Adding to the overhead space required for a cryo-SNOM is the atomic force microscopy (AFM) control, which predominantly utilizes a laser-based detection scheme for determining the cantilever tapping motion. Here we provide an alternative and simplified route for performing s-SNOM using metal-coated Akiyama probes, where the cantilever tapping motion is detected through a piezoelectric signal. The Akiyama-based cryo-SNOM attains high spatial resolution, good near-field contrast, and can perform imaging with a significantly more compact system compared to other cryo-SNOM techniques. By combining this system with a 7 T magnetic field, we have directly imaged Dirac magnetoplasmons in charge-neutral monolayer graphene with subwavelength resolution. These magnetoplasmons manifest as edge interference patterns in the optical signal and as interesting edge currents in the photocurrent signal.

*Stony Brook University authors acknowledge support from the National Science Foundation under Grant No. DMR-1904576. A. G. acknowledges support from the DOE Early Career Research program (Grant 2005410), from the Yale West Campus Materials Characterization Core for SEM imaging of AFM tips and from Attocube Systems in the design of a custom LT-AFM system based on Akiyama probe. M.K.L. acknowledges support from the NSF Faculty Early Career Development Program under Grant No. DMR - 2045425. L. W., X.Z.C, M.K.L., and D.N.B. acknowledge support from the U.S. Department of Energy, Office of Science, Co-design Center for Quantum Advantage (C2QA) under contract number DE-SC0012704. M.D., M.K.L., and Q.L are supported by the U.S. Department of Energy, Division of Materials Sciences and Engineering, under Contract No. DE-SC0012704.Research on m-SNOM design is supported as part of Programmable Quantum Materials, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), under award DE-SC0019443.

Presenters

  • Michael Dapolito

    • Columbia University

Authors

  • Michael Dapolito

    • Columbia University
  • Makoto Tsuneto

    • Stony Brook University
  • Wenjun Zheng

    • Stony Brook University
  • Lukas Wehmeier

    • Brookhaven National Laboratory
  • Suheng Xu

    • Columbia University
  • Xinzhong Chen

    • Stony Brook University (SUNY)
  • Jiacheng Sun

    • Stony Brook University (SUNY)
  • Zengyi Du

    • Brookhaven National Lab.
    • Stony Brook University
  • Zengyi Du

    • Brookhaven National Lab.
    • Stony Brook University
  • Yinming Shao

    • Columbia University
    • Department of Physics, Columbia University, New York, NY, USA
  • Ran Jing

    • Columbia University
  • Shuai Zhang

    • Columbia University
    • Department of Physics, Columbia University, New York, NY, USA
  • Yinan Dong

    • Columbia University
  • Dorri Halbertal

    • Columbia Univ
  • Zijian Zhou

    • Stony Brook University
  • Adrian Gozar

    • Yale University
  • G.Lawrence Carr

    • Brookhaven National Laboratory
  • Michael M Fogler

    • University of California, San Diego
  • Alexey B Kuzmenko

    • Université de Genève
  • Qiang Li

    • Stony Brook University (SUNY)
  • Dmitri N Basov

    • Columbia University
    • Department of Physics, Columbia University, New York, NY, USA
  • Xu Du

    • Stony Brook University (SUNY)
    • Stony Brook University
  • Mengkun Liu

    • Stony Brook University (SUNY)