Noncoplanar Spin Textures in Cubic Double Perovskites Ba<sub>2</sub>YRuO<sub>6</sub> and Ba<sub>2</sub>LuRuO<sub>6</sub>

ORAL

Abstract

Magnetic materials with noncoplanar magnetic structures can show unusual physical properties driven by nontrivial topology. Topologically-active states are often multi-q structures, which are challenging to stabilize in models and to identify in materials. In this talk, we use inelastic neutron-scattering data to show that the insulating double perovskites Ba2YRuO6 and Ba2LuRuO6 -- previously assumed to be collinear antiferromagnets -- actually host a noncoplanar triple-q structure on the face-centered cubic lattice. I discuss the magnetic interactions that may stabilize this state, considering biquadratic exchange and cubic anisotropy. Our work identifies cubic double perovskites as a promising class of materials to realize topological magnetic states, elucidates the likely stabilization mechanism of the triple-q state in these materials, and establishes neutron spectroscopy on powder samples as a valuable technique to distinguish multi-q from single-q structures, facilitating the discovery of topologically-nontrivial magnetic materials.

*This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. It used resources at the Spallation Neutron Source, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory.

Presenters

  • Joe Paddison

    • Oak Ridge National Lab
    • Oak Ridge National Laboratory

Authors

  • Joe Paddison

    • Oak Ridge National Lab
    • Oak Ridge National Laboratory
  • Jiaqiang Yan

    • Oak Ridge National Laboratory
    • Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
  • Hao Zhang

    • University of Tennessee
  • Seunghwan Do

    • Oak Ridge National Laboratory
  • Shang Gao

    • Oak Ridge National Laboratory
    • Department of Physics, University of Science and Technology of China
  • Matthew B Stone

    • Oak Ridge National Lab
    • Oak Ridge National Laboratory
  • David A Dahlbom

    • University of Tennessee
    • University of Tennessee, Knoxville
  • Kipton M Barros

    • Los Alamos Natl Lab
    • Theoretical Division and CNLS, Los Alamos National Laboratory
  • Cristian Batista

    • University of Tennessee
    • University of Tennessee, Knoxville
  • Andy Christianson

    • Oak Ridge National Laboratory
    • Oak Ridge National Lab