Noncoplanar Spin Textures in Cubic Double Perovskites Ba<sub>2</sub>YRuO<sub>6</sub> and Ba<sub>2</sub>LuRuO<sub>6</sub>
ORAL
Abstract
Magnetic materials with noncoplanar magnetic structures can show unusual physical properties driven by nontrivial topology. Topologically-active states are often multi-q structures, which are challenging to stabilize in models and to identify in materials. In this talk, we use inelastic neutron-scattering data to show that the insulating double perovskites Ba2YRuO6 and Ba2LuRuO6 -- previously assumed to be collinear antiferromagnets -- actually host a noncoplanar triple-q structure on the face-centered cubic lattice. I discuss the magnetic interactions that may stabilize this state, considering biquadratic exchange and cubic anisotropy. Our work identifies cubic double perovskites as a promising class of materials to realize topological magnetic states, elucidates the likely stabilization mechanism of the triple-q state in these materials, and establishes neutron spectroscopy on powder samples as a valuable technique to distinguish multi-q from single-q structures, facilitating the discovery of topologically-nontrivial magnetic materials.
*This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. It used resources at the Spallation Neutron Source, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory.
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Presenters
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Joe Paddison
- Oak Ridge National Lab
- Oak Ridge National Laboratory