Valley-coherent quantum anomalous Hall state in AB-stacked MoTe2/WSe2 bilayers

ORAL

Abstract

Moire´ materials provide fertile ground for the correlated and topological quantum phenomena. Among them, the quantum anomalous Hall (QAH) effect, in which the Hall resistance is quantized even under zero magnetic field, is a direct manifestation of the intrinsic topological properties of a material and an appealing attribute for low-power electronics applications. The QAH effect has been observed in both graphene and transition metal dichalcogenide (TMD) moire´ materials. It is thought to arise from the interaction-driven valley polarization of the narrow moire´ bands. Here, we show surprisingly that the newly discovered QAH state in AB-stacked MoTe2/WSe2 moire´ bilayers is not valley-polarized but valley-coherent. The layer- and helicity-resolved optical spectroscopy measurement reveals that the QAH ground state possesses spontaneous spin (valley) polarization aligned (anti-aligned) in two TMD layers. In addition, saturation of the out-of-plane spin polarization in both layers occurs only under high magnetic fields, supporting a canted spin texture. Our results call for a new mechanism for the QAH effect and highlight the potential of TMD moire´ materials with strong electronic correlations and spin-orbit interactions for exotic topological states.

Presenters

  • Zui Tao

    • Cornell University

Authors

  • Zui Tao

    • Cornell University
  • Bowen Shen

    • Cornell University
  • Shengwei Jiang

    • Shanghai Jiaotong university
  • Tingxin Li

    • Shanghai Jiao Tong University
    • Shanghai Jiaotong University
  • Lizhong Li

    • Cornell University
  • Liguo Ma

    • Fudan Univ
    • Cornell University
  • Wenjin Zhao

    • Cornell University, Kavli Institute at Cornell
  • Jenny Hu

    • Stanford University
    • Stanford Univ
  • Kateryna Pistunova

    • Stanford Univ
  • Kenji Watanabe

    • National Institute for Materials Science
    • Research Center for Functional Materials, National Institute of Materials Science
    • Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-044, Japan
    • NIMS
    • Research Center for Functional Materials, National Institute for Materials Science
    • National Institute for Materials Science, Japan
    • Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Japan
    • NIMS Japan
  • Takashi Taniguchi

    • National Institute for Materials Science
    • Kyoto Univ
    • International Center for Materials Nanoarchitectonics, National Institute of Materials Science
    • Kyoto University
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-044, Japan
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • National Institute for Materials Science, Japan
    • National Institute For Materials Science
    • NIMS
    • National Institute for Material Science
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science, Tsukuba, Japan
    • NIMS Japan
  • Tony F Heinz

    • Stanford University
    • SLAC National Accelerator Laboratory
  • Kin Fai Mak

    • Cornell University
  • Jie Shan

    • Cornell University