High Resolution Polar Kerr Effect Studies of CsV3Sb5
ORAL
Abstract
We report high resolution polar Kerr effect measurements on CsV3Sb5 single crystals in search for signatures of spontaneous time reversal symmetry breaking below the charge order transition at T* = 94 K. Utilizing two different versions of zero-area loop Sagnac interferometers operating at 1550 nm wavelength, each with the fundamental attribute that without a time reversal symmetry breaking sample at its path, the interferometer is perfectly reciprocal, we find no observable Kerr effect to within the noise floor limit of the apparatus at 30 nanoradians. Simultaneous coherent reflection ratio measurements confirm the sharpness of the charge order transition in the same optical volume as the Kerr measurements. At finite magnetic field we observe a sharp onset of a diamagnetic shift in the Kerr signal at T*, which persists down to the lowest temperature without change in trend. Since 1550 nm is an energy that was shown to capture all features of the optical properties of the material that interact with the charge order transition, we are led to conclude that it is highly unlikely that time reversal symmetry is broken in the charge ordered state in CsV3Sb5.
*Work at Stanford University was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract DE-AC02-76SF00515. Work at UC Irvine was supported by the Gordon and Betty Moore Foundation through Grant GBMF10276. S.D.W. and B.R.O. acknowledge support via the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under award DMR-1906325. R.T. acknowledges support from the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) through QUAST FOR 5249-449872909 (Project P3), through Project-ID 258499086-SFB 1170, and from the Würzburg-Dresden Cluster of Excellence on Complexity and Topology in Quantum Matter – ct.qmat Project-ID 390858490-EXC 2147.
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Publication:David R. Saykin, Camron Farhang, Erik D. Kountz, Dong Chen, Brenden R. Ortiz, Chandra Shekhar, Claudia Felser, Stephen D. Wilson, Ronny Thomale, Jing Xia, Aharon Kapitulnik High Resolution Polar Kerr Effect Studies of CsV3Sb5: Tests for Time Reversal Symmetry Breaking Below the Charge Order Transition https://arxiv.org/abs/2209.10570
Presenters
David Saykin
Stanford University
Authors
David Saykin
Stanford University
Camron Farhang
University of California, Irvine
Erik D Kountz
Stanford University
Dong Chen
Max Planck Institute for Chemical Physics of Solids
Brenden Ortiz
University of California, Santa Barbara
Chandra Shekhar
Max Planck Institute for Chemical Physics of Solids
Claudia Felser
Max Planck Institute for Chemical Physic
Max Planck Institute for Chemical Physics of Solids
Stephen D Wilson
Materials Department, University of California Santa Barbara
University of California, Santa Barbara
UCSB
Ronny Thomale
Julius-Maximilians University of Wuerzburg
Julius-Maximilians University of Wuerzbu
Institut für Theoretische Physik und Astrophysik Universität Würzburg, 97074 Würzburg, Germany