Flexomagnetism of thin Cr<sub>2</sub>O<sub>3</sub> films

ORAL

Abstract

Cr2O3 is the only known uniaxial antiferromagnetic material that is also magnetoelectric at room temperature. This renders Cr2O3 a technologically relevant playground for the realisation of different device ideas for prospective antiferromagnetic spintronics. We discovered the presence of flexomagnetic effects in Cr2O3, which come about due to the impact of a strain gradient on the thermodynamic properties, namely on the Neel temperature. By combining magnetotransport and Nitrogen Vacancy magnetometry characterizations, we experimentally determine the presence of the gradient of the Neel temperature in a 50-nm-thick Cr2O3 thin film and quantify that the magnetic moment, generated by this new effect, can be as high as 15 μB/nm2. Furthermore, due to good oxide-oxide heteroepitaxy and respective compressive strain, the Neel temperature in Cr2O3 thin films can be enhanced persistently up to 100 °C, which is 60 °C higher than the bulk transition temperature. The emergent flexomagnetism-driven ferromagnetic order parameter in antiferromagnetic thin films offers more flexibility in the design of spintronic and magnonic devices and can be of relevance for other antiferromagnetic materials.

Publication: P. Makushko, T. Kosub, O. V. Pylypovskyi et al., Nature Communications (2022), in press.

Presenters

  • Oleksandr V Pylypovskyi

    • Helmholtz Zentrum Dresden-Rossendorf
    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research

Authors

  • Oleksandr V Pylypovskyi

    • Helmholtz Zentrum Dresden-Rossendorf
    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Pavlo Makushko

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Tobias Kosub

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Natascha Hedrich

    • University of Basel
  • JIang Li

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Alexej Pashkin

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Stanislav Avdoshenko

    • Institute for Solid State Research, Leibniz Institute for Solid State and Materials Research Dresden
  • Rene Hübner

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Fabian Ganss

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Daniel Wolf

    • IFW Dresden, Germany
    • Institute for Solid State Research, IFW Dresdenm Dresden, Germany
    • Leibniz Institute for Solid State and Materials Research, IFW Dresden
  • Axel Lubk

    • Institute for Solid State Research, IFW Dresdenm Dresden, Germany
    • Leibniz Institute for Solid State and Materials Research, IFW Dresden
  • Maciej Oskar Liedke

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Radiation Physics
  • Maik Butterling

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Radiation Physics
  • Andreas Wagner

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Radiation Physics
  • Kai Wagner

    • University of Basel
  • Brendan Shields

    • University of Basel
  • Paul Lehmann

    • University of Basel
  • Ihor Veremchuk

    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Jürgen Fassbender

    • Helmholtz-Zentrum Dresden-Rossendorf
    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Dresden, Germany
    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research
  • Patrick Maletinsky

    • University of Basel
  • Denys Makarov

    • Helmholtz-Zentrum Dresden-Rossendorf
    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Dresden, Germany
    • Helmholtz-Zentrum Dresden-Rossendorf e.V., Institute of Ion Beam Physics and Materials Research