Effects of anti-site defect-induced disorder in compensated topological magnet MnBi<sub>1.36</sub>Sb<sub>0.64</sub>Te<sub>4</sub>

ORAL

Abstract

The gapped Dirac-like surface states of magnetic topological insulator MnBi2-xSbxTe4 (MBST) are a promising host for exotic quantum phenomena such as the quantum anomalous Hall effect and axion insulating states. However, it has become clear that atomic defects undermine the stabilization of such quantum phases as they lead to spatial variations in the surface state gap and doping levels. The large number of possible defect configurations in MBST make studying the influence of individual defects virtually impossible. Here, we present a statistical analysis of the nanoscale effect of defects in MBST by scanning tunneling microscopy/spectroscopy (STM/S). We identify (Bi,Sb)Mn anti-site defects to be the main source of doping fluctuations, resulting in the formation of nanoscale charge puddles, while Mn(Bi/Sb) anti-site defects are the main source of fluctuations in the surface state gap. Our findings can guide further optimization of this material system via defect engineering.

*This work was supported by Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy (DOE), Office of Science User Facility at Oak Ridge National Laboratory.

Publication: arXiv preprint arXiv:2208.13374

Presenters

  • An-Ping Li

    • Oak Ridge National Lab

Authors

  • An-Ping Li

    • Oak Ridge National Lab
  • Felix Luepke

    • Oak Ridge National Laboratory
  • Marek Kolmer

    • Oak Ridge National Laboratory
  • Jiaqiang Yan

    • Oak Ridge National Laboratory
    • Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
  • Hao Chang

    • Oak Ridge National Laboratory
  • Paolo Vilmercati

    • University of Tennessee
  • Hanno H Weitering

    • University of Tennessee
  • Wonhee Ko

    • University of Tennessee, Knoxville
    • Department of Physics and Astronomy, University of Tennessee at Knoxville, Knoxville TN 37996, USA
    • University of Tennessee