Nonlinear and Quantum Semiconductor Metasurface

ORAL  · Invited

Abstract

Metamaterials and their 2D implementation – metasurfaces - have been used extensively for wavefront manipulation since their inception nearly two decades ago. This has led to a revolution in optics due to the ability to design optical components with functionality and form factor that was unthinkable not long ago. Another use of metasurfaces relies on the ability to tailor distributions and intensities of local electromagnetic fields to study a variety of fundamental phenomena in light-matter interaction, create novel tunable and active devices and enhance optical nonlinearities.



In the context of quantum and nonlinear optics, III-V semiconductors have among the highest optical nonlinearities but cannot be used in conventional phase-matched processes due to the symmetry of their nonlinear susceptibility tensor. However, as phase matching is relaxed when resonant nanoscale resonators are used, III-V semiconductor metasurfaces can be used for harmonic generation, harmonic mixing and parametric down-conversion in ways that have no equivalence when using macroscopic nonlinear media. Some of the results that I’ll present include harmonic generation and generation of entangled photons and complex quantum states using spontaneous parametric down-conversion enabled by quasi bound-states in the continuum resonances.



*Work supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (grant BES 20-017574). The work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the US Department of Energy, Office of Science. Sandia National Laboratories is a multi-mission laboratory managed and operated by National Technology and Engineering Solutions of Sandia LLC, a wholly owned subsidiary of Honeywell International Inc., for the US Department of Energy's National Nuclear Security Administration under contract DE-NA0003525. This paper describes objective technical results and analysis. Any subjective views or opinions that might be expressed in the paper do not necessarily represent the views of the US Department of Energyor the United States government.

Publication: 1. "An All-Dielectric Polaritonic Metasurface with a Giant Nonlinear Optical Response", R. Sarma, J. Xu, D. de Ceglia, L. Carletti, S. Campione, J. Klem, M. B. Sinclair, M. A. Belkin and I. Brener, Nano Lett 22, 896 (2022). DOI: 10.1021/acs.nanolett.1c03325
2. "Resonant metasurfaces for generating complex quantum states", T. Santiago-Cruz, S. D. Gennaro, O. Mitrofanov, S. Addamane, J. Reno, I. Brener and M. V. Chekhova, Science 377, 991 (2022). DOI: 10.1126/science.abq8684
3. "Cascaded Optical Nonlinearities in Dielectric Metasurfaces", S. D. Gennaro, C. F. Doiron, N. Karl, P. P. Iyer, D. K. Serkland, M. B. Sinclair and I. Brener, Acs Photonics 9, 1026 (2022). DOI: 10.1021/acsphotonics.1c01937
4. "Nonlinear and ultrafast all-dielectric metasurfaces at the center for integrated nanotechnologies", S. Gennaro, R. Sarma and I. Brener, Nanotechnology 33 (2022). DOI: 10.1088/1361-6528/ac7654

Presenters

  • Igal Brener

    • Sandia National Laboratories

Authors

  • Igal Brener

    • Sandia National Laboratories