Intriguing Magnetism of the Topological Kagome Magnet TbMn<sub>6</sub>Sn<sub>6</sub>

ORAL

Abstract

Magnetic topological phases of quantum matter are an emerging frontier in physics and material science [1-3], of which kagome magnets appear as a highly promising platform. Here, we explore magnetic correlations in the recently identified topological kagome system TbMn6Sn6 using muon spin rotation, combined with local field analysis and neutron diffraction [1]. Our studies identify an out-of-plane ferrimagnetic structure with slow magnetic fluctuations which exhibit a critical slowing down below T*C1 ≅ 120 K and finally freeze into static patches with ideal out-of-plane order below TC1 ≅ 20 K. The appearance of the static patches sets in at a similar temperature as the topological transport behaviors. We further show that a hydrostatic pressure of 2.1 GPa stabilizes the static out-of-plane topological ferrimagnetic ground state in the whole volume of the sample. Therefore the exciting perspective arises of a magnetically-induced topological system whose magnetism can be controlled through external control parameters. The present results [1] will stimulate theoretical investigations to obtain a microscopic understanding of the relation between the low-temperature volume-wise magnetic evolution of the static c-axis ferrimagnetic patches and the topological electronic properties in TbMn6Sn6.



[1] C. Mielke III et al., Comm. Phys. 5, 107 (2022).

[2] J.-X. Yin et al., Nature 583, 533-536 (2020).

[3] N.J. Ghimire and I.I. Mazin, Nature Materials 19, 137-138 (2020).

Publication: C. Mielke III et al. Low-temperature magnetic crossover in the topological kagome magnet TbMn6Sn6. Communications Physics 5, 107 (2022).

Presenters

  • Charles Mielke

    • University of Zurich

Authors

  • Charles Mielke

    • University of Zurich
  • Zurab Guguchia

    • Paul Scherrer Institute
    • Paul Scherrer Institut
  • Wenlong Ma

    • International Center for Quantum Materials, School of Physics, Peking University, Beijing, China
  • Vladimir Pomjakushin

    • Paul Scherrer Institut, Switzerland
    • Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut, CH-5232, Villigen, PSI, Switzerland
  • Oksana Zaharko

    • Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institute, CH-5232 Villigen, Switzerland
    • Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut, CH-5232, Villigen, PSI, Switzerland
  • Simone Sturniolo

    • Scientific Computing Department, Science & Technology Facilities Council UKRI, Rutherford Appleton Laboratory, Harwell Campus, Didcot, OX11 0QX, UK
  • Victor Ukleev

    • Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institut, CH-5232, Villigen, PSI, Switzerland
  • Jonathan S White

    • Paul Scherrer Institute
  • Jiaxin Yin

    • Princeton University
  • Stepan S Tsirkin

    • Univ of Zurich
  • Tyler A Cochran

    • Princeton University
  • Marisa Medarde

    • Laboratory for Multiscale Materials Experiments, Paul Scherrer Institut, CH-5232, Villigen, PSI, Switzerland
  • Victor Porée

    • Paul Scherrer Institut
  • Debarchan Das

    • Paul Scherrer Institute
    • Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232, Villigen, PSI, Switzerland
    • LMU, Paul Scherrer Institute, Switzerland
  • Ritu Gupta

    • Paul Scherrer Institute
    • Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232, Villigen, PSI, Switzerland
  • Johan Chang

    • University of Zürich
    • Department of Physics, University of Zürich, Winterthurerstrasse 190, Zurich, Switzerland
    • University of Zurich
  • Zhi-Cheng Wang

    • Boston College
  • Rustem Khasanov

    • Paul Scherrer Institute
    • Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232, Villigen, PSI, Switzerland
  • Titus Neupert

    • Univ of Zurich
  • Alex Amato

    • Paul Scherrer Institute
    • Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232, Villigen, PSI, Switzerland
  • Leandro Liborio

    • Scientific Computing Department, Science & Technology Facilities Council UKRI, Rutherford Appleton Laboratory, Harwell Campus, Didcot, OX11 0QX, UK
  • Hubertus Luetkens

    • Paul Scherrer Institute
    • Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute, CH-5232, Villigen, PSI, Switzerland
  • Shuang Jia

    • Peking Univ