Coherent charge carrier dynamics in the presence of thermal lattice vibrations

ORAL

Abstract

We develop the coherent state representation of lattice vibrations to describe their interactions with charge carriers. In direct analogy to quantum optics, the coherent state representation leads from quantized lattice vibrations (phonons) naturally to a quasiclassical field limit, i.e., the deformation potential. To an electron, the deformation field is a sea of hills and valleys, as ``real'' as any external field, morphing and propagating at the sound speed, and growing in magnitude with temperature. In this disordered potential landscape, the charge carrier dynamics is treated nonperturbatively, preserving their coherence beyond single collision events. We show the coherent state picture agrees exactly with the conventional Fock state picture in perturbation theory. Furthermore, it goes beyond by revealing aspects that the conventional theory could not explain: transient localization even at high temperatures by charge carrier coherence effects, and band tails in the density of states due to the self-generated disorder (deformation) potential in a pure crystal. The coherent state paradigm of lattice vibrations supplies tools for probing important questions in condensed matter physics as in quantum optics.

*We thank the National Science Foundation for supporting this research, through the NSF the Center for Integrated Quantum Materials (CIQM) Grant No. DMR-1231319. A.A. acknowledges support from The Scientific and Technological Research Council of Turkey (T"urkiye Bilimsel ve Teknolojik Arac{s}t{i}rma Kurumu, T"UB.{I}TAK) Program Code 2219. J.K.-R. thanks the Emil Aaltonen Foundation for financial support.

Publication: Phys. Rev. B 106, 054311 (2022)

Presenters

  • Donghwan Kim

    • Harvard University

Authors

  • Donghwan Kim

    • Harvard University
  • Alhun Aydin

    • Harvard University
    • Harvard University, Koc University
    • Koç University
  • Alvar Daza

    • Universidad Rey Juan Carlos
  • Kobra N Avanaki

    • Harvard University
  • Joonas Keski-Rahkonen

    • Harvard University
  • Eric J Heller

    • Harvard University