Controlling magnetic configuration in soft-hard bilayers probed by polarized neutron reflectometry

Hard/soft magnetic bilayer thin films have been widely used in data storage technologies and permanent magnet applications. The magnetic configuration and response to temperatures and magnetic fields in these heterostructures are considered to be highly dependent on the interfacial coupling. However, the intrinsic properties of each of the layers, such as the saturation magnetization and layer thickness, also strongly influence the magnetic configuration. Changing these parameters provides an effective method to tailor magnetic properties in composite magnets. Here, we use polarized neutron reflectometry (PNR) to experimentally probe the interfacial magnetic configurations in hard/soft bilayer thin films: L1₀-FePt/A1-FePt, [Co/Pd] /CoPd, [Co/Pt] /FeNi and L1₀-FePt/Fe at room temperature, which all have a perpendicular magnetic anisotropy in the hard layer. These films were designed with different soft and hard layer thicknesses ( and ) and saturation magnetization ( and ), respectively. The influences of an in-plane magnetic field () and temperature (T) are also studied using a L1₀‑FePt/A1-FePt bilayer sample. Comparing the PNR results to micromagnetic simulations reveals that the interfacial magnetic configuration is highly dependent on ,  and the external factors ( and T), and has a relatively weak dependence on  and . Key among these results, for thin , the hard and soft layers are rigidly coupled in the out-of-plane direction, then undergo a transition to relax in-plane. This transition can be delayed to larger  by decreasing  Understanding the influence of these parameters on the magnetic configuration is critical to designing functional composite magnets for applications.