Nano-optical imaging of localization phenomena in low-angle twisted bilayer graphene.

POSTER

Abstract

We present evidence for lattice localization physics in the novel reconstructed twisted bilayer graphene (rTBG) system. Here, two graphene layers with an angle smaller than one degree produce the rTBG. In this condition, the carbon atoms rearrange, forming triangular structures composed of solitons and topological points. We use nano-Raman spectroscopy, where a visible-light laser beam is focused on a nano-antenna, to image the rTBG structure. In addition to the first crystalline structure visualization by visible light, this technique provides in-depth spectroscopic information of the rTBG system. Thus, we observe the manifestation of the non-conventional localization of phonons and the already predicted electronic localization. Besides, we also illustrate that the electron-phonon coupling in this system is unique, and its understanding can help elucidate the magic-angle superconductivity. Therefore, our work unravels fascinating phenomena in the fast-developing twistronics field.

*This work was supported by CNPq (302775/2018-8 and INCT/Nanomaterials de Carbono), CAPES (RELAII and 88881.198744/2018-01) and FAPEMIG, Brazil. V.-H.N. and J.-C.C. acknowledge financial support from the Fédération Wallonie-Bruxelles through the ARC on 3D nano-architecturing of 2D crystals (16/21-077), from the European Union's Horizon 2020 Research Project and Innovation Program — Graphene Flagship Core3 (881603), from the Flag-Era JTC projects 'MECHANIC' (R.50.07.18) and 'TATTOOS' (R.8010.19), from the Belgium FNRS through the research projects T.1077.15 and T.0051.18, and from the Francqui-Stichting Foundation. V.M. and M.L. acknowledge support from NY State Empire State Development's Division of Science, Technology and Innovation (NYSTAR).

Publication: Nature volume 590, pages405–409 (2021)
arXiv:2006.09482
2D Mater. 8 035046 (2021)

Presenters

  • Andreij Gadelha

    • University of Colorado, Boulder

Authors

  • Andreij Gadelha

    • University of Colorado, Boulder