Lumped element superconducting resonators for electrical control and read-out of molecular spin qubits

ORAL

Abstract

Paramagnetic molecular spin systems strongly coupled to superconducting resonators are promising building blocks for hybrid quantum processors. However, the control of specific operations remains a challenge as the spin coherence times are not yet sufficiently long as compared with the coupling rate. Our approach is to electrically control and read-out the spin state of a high-spin (S = 5/2) paramagnetic manganese(II) molecules embedded in its polar piezoelectric diamagnetic Zn(II) host lattice. We have developed lumped-element resonators (LERs) that, through the resonant microwave fields, modify the local ion coordination modulating the magnetic anisotropy that determines the spin qubit Hamiltonian and transition rates. The use of superconducting microwave resonators implies low losses, high-quality factors and multiplexability which are crucial for this application permitting the simultaneous readout of several qubits. M. C. de Ory and S. Roca contributed equally to this work.

*We acknowledge support from EU (FETOPEN-RIA-2019-01 862893, QUANTERA SUMO), Spanish MCIU/AEI/FEDER (PID2019-105552RB-41, RTI-2018-096075-B-C21, PCI2018-093116 and PID2019-105552RB-44), ONR-Global (DEFROST N62909-19-1-2053), French ANR project SMolMagIQ (ANR-20-CE29-0010) and CSIC Research Platform PTI-001.

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Presenters

  • Marina C de Ory

    • Spanish National Research Council (CSIC) / Spanish National Institute of Aerospace Technology (INTA)
    • Centro de Astrobiología CSIC-INTA, 28850 Torrejón de Ardoz, Spain
    • Spanish National Research Council (CSIC)

Authors

  • Marina C de Ory

    • Spanish National Research Council (CSIC) / Spanish National Institute of Aerospace Technology (INTA)
    • Centro de Astrobiología CSIC-INTA, 28850 Torrejón de Ardoz, Spain
    • Spanish National Research Council (CSIC)

  • Sebastián Roca

    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.

  • Marcos Rubin-Osanz

    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.
    • Consejo Superior de Investigaciones Cientificas (CSIC) / Universidad de Zaragoza / INMA
    • Spanish National Research Council (CSIC)

  • Victor Rollano

    • Spanish National Research Council (CSIC) / University of Zaragoza
    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.

  • María Teresa Magaz

    • Centro de Astrobiología CSIC-INTA, 28850 Torrejón de Ardoz, Spain

  • Daniel Granados

    • IMDEA Nanociencia, Calle Faraday 9, Campus de Cantoblanco, 28049 Madrid, Spain
    • IMDEA Nanoscience

  • David Zueco

    • Spanish National Research Council (CSIC) / University of Zaragoza
    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.
    • Consejo Superior de Investigaciones Cientificas (CSIC)
    • Consejo Superior de Investigaciones Cientificas (CSIC) / Universidad de Zaragoza / INMA
    • Spanish National Research Council (CSIC)

  • François Lambert

    • Institut de Chimie Moléculaire et des Matériaux d'Orsay, CNRS, Université Paris-Saclay, 15, rue Georges Clemenceau, 91405 Orsay Cedex, France

  • Talal Mallah

    • French National Centre for Scientific Research (CNRS) / Paris-Saclay University
    • Institut de Chimie Moléculaire et des Matériaux d'Orsay, CNRS, Université Paris-Saclay, 15, rue Georges Clemenceau, 91405 Orsay Cedex, France

  • Fernando M Luis

    • INMA(CSIC-U. Zaragoza)
    • Spanish National Research Council (CSIC) / University of Zaragoza
    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.
    • Instituto de Nanociencia y Materiales de Aragón (CSIC-Universidad de Zaragoza)
    • Consejo Superior de Investigaciones Cientificas (CSIC) / Universidad de Zaragoza / INMA
    • Spanish National Research Council (CSIC)

  • Alicia Gomez

    • Spanish National Research Council (CSIC) / Spanish National Institute of Aerospace Technology (INTA)
    • Centro de Astrobiología CSIC-INTA, 28850 Torrejón de Ardoz, Spain
    • Spanish National Research Council (CSIC)