Probing nematicity and magnetism with combined tunable strain and x-ray scattering/fluorescence techniques
ORAL · Invited
Abstract
In this talk I will review our recent progress at the Advanced Photon Source in combining in situ tunable uniaxial stress with simultaneous transport measurements and several synchrotron x-ray techniques to perform unique characterizations of several iron-based superconductors. In Co-doped BaFe2As2 we use x-ray diffraction (XRD) to carefully monitor the strain detwinning of the orthorhombic structural domains and make a precise determination of the spontaneous resistivity anisotropy across temperature within the nematic phase. In EuFe2As2 we use x-ray magnetic circular dichroism (XMCD) to make the first observation of a magnetic field-induced spin flip transition of antiferromagnetic Eu moments in a strain-detwinned sample. In Co-doped EuFe2As2 we use XMCD to monitor the magnetic field-induced reorientation of ferromagnetic Eu moments from out of plane to in-plane, which we correlate with a strain-tunable field-induced superconductivity. Finally, in FeSe we combine XRD and x-ray linear dichroism (XLD) to observe the nematic orbital polarization anisotropy within the nematic phase across a range of strain and detwinning values. This unique combination of tuning and probing techniques has so far given new insight into these interesting materials and presents a new approach to answering unresolved questions in iron-based superconductors and beyond.
*J.J. Sanchez acknowledges support from the Department of Energy SCGSR Program administered by ORISE, and from the National Science Foundation MPS-Ascend Program.
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Publication:J.J. Sanchez et al. "The transport–structural correspondence across the nematic phase transition probed by elasto X-ray diffraction". Nature Materials 20, 1519-1524 (2021) J.J. Sanchez et al. "Strongly anisotropic antiferromagnetic coupling in EuFe2As2 revealed by stress detwinning". Physical Review B 104, 10 (2021) J.J. Sanchez et al. "Strain-switchable field-induced superconductivity". In preparation (2022) J.J. Sanchez and C. Occhialini et al. "Spontaneous orbital anisotropy in the nematic phase of FeSe probed by elasto X-ray linear dichroism". In preparation (2022)
Presenters
Joshua J Sanchez
Massachusetts Institute of Technology
University of Washington
University of Washington / MIT
Authors
Joshua J Sanchez
Massachusetts Institute of Technology
University of Washington
University of Washington / MIT
Connor A Occhialini
Massachusetts Institute of Technology
Massachusetts Institute of Technology MIT
Massachusetts Institute of Technology MI
Philip J Ryan
Argonne National Laboratory
Jong Woo Kim
Argonne National Laboratory
Advanced Photon Source, Argonne National Laboratory
Gilberto F Fabbris
Argonne National Laboratory
Yongseong Choi
Argonne National Laboratory
Argonne National Lab
Jian Liu
University of Tennessee
Shashi K Pandey
University of Tennessee
Paul T Malinowski
University of Washington
Yue Shi
University of Washington
Jiun-Haw Chu
University of Washington
Igor Mazin
George Mason University
Department of Physics and Astronomy and Quantum Science and Engineering Center, George Mason University, Fairfax, Virginia 22030, USA
Quantum Science and Engineering Center, Department of Physics and Astronomy - George Mason University