Probing nematicity and magnetism with combined tunable strain and x-ray scattering/fluorescence techniques

ORAL  · Invited

Abstract

In this talk I will review our recent progress at the Advanced Photon Source in combining in situ tunable uniaxial stress with simultaneous transport measurements and several synchrotron x-ray techniques to perform unique characterizations of several iron-based superconductors. In Co-doped BaFe2As2 we use x-ray diffraction (XRD) to carefully monitor the strain detwinning of the orthorhombic structural domains and make a precise determination of the spontaneous resistivity anisotropy across temperature within the nematic phase. In EuFe2As2 we use x-ray magnetic circular dichroism (XMCD) to make the first observation of a magnetic field-induced spin flip transition of antiferromagnetic Eu moments in a strain-detwinned sample. In Co-doped EuFe2As2 we use XMCD to monitor the magnetic field-induced reorientation of ferromagnetic Eu moments from out of plane to in-plane, which we correlate with a strain-tunable field-induced superconductivity. Finally, in FeSe we combine XRD and x-ray linear dichroism (XLD) to observe the nematic orbital polarization anisotropy within the nematic phase across a range of strain and detwinning values. This unique combination of tuning and probing techniques has so far given new insight into these interesting materials and presents a new approach to answering unresolved questions in iron-based superconductors and beyond.

*J.J. Sanchez acknowledges support from the Department of Energy SCGSR Program administered by ORISE, and from the National Science Foundation MPS-Ascend Program.

Publication: J.J. Sanchez et al. "The transport–structural correspondence across the nematic phase transition probed by elasto X-ray diffraction". Nature Materials 20, 1519-1524 (2021)
J.J. Sanchez et al. "Strongly anisotropic antiferromagnetic coupling in EuFe2As2 revealed by stress detwinning". Physical Review B 104, 10 (2021)
J.J. Sanchez et al. "Strain-switchable field-induced superconductivity". In preparation (2022)
J.J. Sanchez and C. Occhialini et al. "Spontaneous orbital anisotropy in the nematic phase of FeSe probed by elasto X-ray linear dichroism". In preparation (2022)

Presenters

  • Joshua J Sanchez

    • Massachusetts Institute of Technology
    • University of Washington
    • University of Washington / MIT

Authors

  • Joshua J Sanchez

    • Massachusetts Institute of Technology
    • University of Washington
    • University of Washington / MIT
  • Connor A Occhialini

    • Massachusetts Institute of Technology
    • Massachusetts Institute of Technology MIT
    • Massachusetts Institute of Technology MI
  • Philip J Ryan

    • Argonne National Laboratory
  • Jong Woo Kim

    • Argonne National Laboratory
    • Advanced Photon Source, Argonne National Laboratory
  • Gilberto F Fabbris

    • Argonne National Laboratory
  • Yongseong Choi

    • Argonne National Laboratory
    • Argonne National Lab
  • Jian Liu

    • University of Tennessee
  • Shashi K Pandey

    • University of Tennessee
  • Paul T Malinowski

    • University of Washington
  • Yue Shi

    • University of Washington
  • Jiun-Haw Chu

    • University of Washington
  • Igor Mazin

    • George Mason University
    • Department of Physics and Astronomy and Quantum Science and Engineering Center, George Mason University, Fairfax, Virginia 22030, USA
    • Quantum Science and Engineering Center, Department of Physics and Astronomy - George Mason University
  • Riccardo Comin

    • Massachusetts Institute of Technology MI
    • Massachusetts Institute of Technology
    • Massachusetts Institute of Technology MIT