Voltage-controlled moiré potentials and long-range propagation of indirect excitons in a van der Waals MoSe<sub>2</sub>/WSe<sub>2</sub> heterostructure

ORAL

Abstract

Excitonic devices based on controlled propagation of indirect excitons (IXs) are demonstrated in GaAs structures but limited to low temperatures due to low IX binding energies [1]. IXs in transition-metal dichalcogenide (TMD) heterostructures are characterized by high binding energies offering the opportunity for room-temperature operation. However, strong moiré superlattice potentials in TMD heterostructures [2,3] localize IXs, making IX propagation different in TMD and GaAs heterostructures. In earlier excitonic devices IX transport was controlled by an energy barrier to IX propagation created by the gate electrode [1]. We present a new mechanism for exciton transport control. It is based on tuning the moiré potentials by voltage to enable IX delocalization. We present the long-range IX propagation due to this mechanism. We also establish a spatial correlation between IX linewidth, energy, and luminescence intensity.

[1] A. A. High et al. Science 321, 229 (2008).

[2] F. Wu et al. PRL 118, 147401 (2017).

[3] H. Yu et al. Sci. Adv. 3, e1701696 (2017).

*These studies were supported by DOE Office of Basic Energy Sciences under award DE-FG02-07ER46449. The heterostructure fabrication and data analysis were supported by NSF grant 1905478.

Publication: L. H. Fowler-Gerace, D. J. Choksy, and L. V. Butov, Voltage-controlled long-range propagation of indirect excitons in a van der Waals heterostructure, Phys. Rev. B 104, 165302 (2021)

Presenters

  • Lewis Fowler-Gerace

    • University of California, San Diego

Authors

  • Lewis Fowler-Gerace

    • University of California, San Diego
  • Zhiwen Zhou

    • University of California, San Diego
  • Darius J Choksy

    • University of California, San Diego
    • University of California at San Diego, La Jolla, California 92093, USA
  • Leonid V Butov

    • University of California, San Diego
    • University of California at San Diego, La Jolla, California 92093, USA