Magnetic field effects on superconductivity near frustrated Mott insulator.

ORAL

Abstract

Quasi-2D organic charge transfer salts are considered model systems for understanding unconventional superconductivity (SC) in cuprates and other correlated electron systems.  However, studies of SC in quasi-2D organics have been limited because the SC phase is typically reached by applying pressure.  In contrast, we perform experiments under ambient pressure on κ-[(BEDT-TTF)0.88(BEDT-STF)0.12]2Cu2(CN)3, which is formed by partial chemical substitution of a quantum spin liquid candidate κ-(BEDT-TTF)2Cu2(CN)3.  We measure linear and nonlinear dc transport over a wide range of perpendicular magnetic fields (H) and temperatures (T) down to ~0.25 K.  The results indicate the onset of SC at ~ 3 K for H=0.  The suppression of SC with H reveals, surprisingly, an insulatinglike normal state.  The underlying field-tuned superconducting quantum phase transition and the nature of the high-field normal state will be discussed and compared to those in cuprates.

*Supported by NSF DMR-1707785, and the NHMFL via NSF DMR-1644779, and the State of Florida.

Publication: Pustogow et al., Nat. Commun. 12, 1571 (2021); Pustogow et al., npj Quantum Mater. 6, 9 (2021); Saito et al., J. Mat. Chem. C 9, 10841 (2021); Saito et al., Crystals 11, 817 (2021).

Presenters

  • Yuxin Wang

    • Dept. of Phys. & Natl. High Magnetic Field Lab., Florida State Univ.
    • Florida State University

Authors

  • Yuxin Wang

    • Dept. of Phys. & Natl. High Magnetic Field Lab., Florida State Univ.
    • Florida State University
  • Dragana Popovic

    • Florida State University
    • Dept. of Phys. & Natl. High Magnetic Field Lab., Florida State Univ.
  • Yohei Saito

    • University of Stuttgart
    • Phys. Inst., Univ. Stuttgart
  • Martin Dressel

    • University of Stuttgart
    • Phys. Inst., Univ. Stuttgart
  • Andrej Pustogow

    • TU Wien, Vienna, Austria
    • Inst. of Solid State Phys., TU Wien
  • Atsushi Kawamoto

    • Hokkaido University, Japan
    • Dept. of Phys., Hokkaido Univ.