Magnetic ordering in Co doped SrNi<sub>2</sub>P<sub>2</sub>.

ORAL

Abstract

SrNi2P2 is an intriguing system as it exhibits fully gapped superconductivity and adopts a unique third-collapsed tetragonal (tcT) phase[1,2]. It transitions from uncollapsed tetragonal (ucT) to tcT phase at T=< 326 K, where only one-third of P atoms bond across the Sr layer. Substituting Ni with Co completely suppresses Ts, drives sytem to ucT phase, and induces various magnetic ground states. The magnetic phase diagram of Sr(Ni1-xCox)2Pobtained from the magnetization measurements shows that even though both stoichiometric SrNi2P2 and SrCo2P2 are paramagnetic, Sr(Ni1-xCox)2Pare antiferromangetic for 0.58<≈x<≈0.94 and ferromagnetic for 0.95<≈x<≈0.98. Single-crystal neutron diffraction measurements performed on = 0.88 sample confirms the long-range antiferromagnetic ordering with helical arrangement of spins along c-direction. Also, feature corresponding to ferromagnetic ordering was observed for x = 0.96. [1] F. Ronning et al PRB 79,134507(2009). [2] S. Xiao et al Nano Lett. 21,7913(2021).

*Work at Ames Laboratory was supported by the U.S. DOE, Office of BES, DMSE. Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. This research used resources at HFIR, a DOE Office of Science User Facility operated by the ORNL.

Presenters

  • Aashish Sapkota

    • Ames Laboratory/Iowa State University
    • Ames Laboratory

Authors

  • Aashish Sapkota

    • Ames Laboratory/Iowa State University
    • Ames Laboratory
  • John M Wilde

    • Iowa State University
    • Iowa State University/Ames Laboratory
  • Juan Schmidt

    • Ames Lab
    • Iowa State University/Ames Laboratory
    • Iowa State University
  • Paul C Canfield

    • Iowa State University
    • Ames Laboratory and Department of Physics, Iowa State University
    • Ames Laboratory/Iowa State University
  • Sergey L Budko

    • Iowa State University
    • Ames Laboratory and Department of Physics, Iowa State University
    • Ames Laboratory/Iowa State University
  • Wei Tian

    • Oak Ridge National Laboratory
    • Oak Ridge National Laboratory, HFIR
    • Oak Ridge National Lab
  • Masaaki Matsuda

    • Oak Ridge National Lab
    • Oak Ridge National Laboratory
  • Guilherme Gorgen Lesseux

    • Iowa State University