Polaronic behavior in La<sub>1.2</sub>Sr<sub>1.8</sub>Mn<sub>2</sub>O<sub>7</sub>

ORAL

Abstract

La1.2Sr1.8Mn2O7 has been an intriguing candidate for probing electronic correlations due to the concomitant emergence of colossal magneto resistance with its paramagnetic-insulating to ferromagnetic-metallic transition at Tc = 120 K. Experimental evidence has demonstrated the relevance of polarons across the phase transition. In particular, early ARPES studies showed the abrupt formation of a small quasi-particle peak with strong mass renormalization in the metal phase which has been associated with a polaronic metal state. Yet, conflicting results revealing finite quasi particle spectral weight even above Tc and combined ARPES/STM studies showing sensitivity to the cleaved surface cast doubt on the polaronic metal scenario. Here we use resonant inelastic X-ray scattering (RIXS) which is a bulk-sensitive two-photon-probe. In contrast to ARPES which measures the single particle spectral function, RIXS probes collective excitations and is thus especially suitable for the investigation of charge-lattice coupled phenomena. In this presentation, we will discuss the RIXS signatures of polarons in La1.2Sr1.8Mn2O7.

*The RIXS experiments were performed at beamline 41A of the Taiwan Photon Source. This work is supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, under contract DE-AC0276SF00515. D.J. acknowledges funding of the Alexander-von-Humboldt foundation via a Feodor-Lynen postdoctoral fellowship.

Presenters

  • Daniel Jost

    • Stanford University
    • SLAC - Natl Accelerator Lab

Authors

  • Daniel Jost

    • Stanford University
    • SLAC - Natl Accelerator Lab
  • Matteo Rossi

    • SLAC - Natl Accelerator Lab
  • Yonghun Lee

    • Stanford University
  • John F Mitchell

    • Argonne National Laboratory
  • Amol Singh

    • Natl Synchrotron Rad Res Ctr
  • Hsiaoyu Huang

    • Natl Synchrotron Rad Res Ctr
    • National Synchrotron Radiation Research Center
  • Di-Jing Huang

    • Natl Synchrotron Rad Res Ctr
  • Zhixun Shen

    • Stanford University
    • Geballe Laboratory for Advanced Materials, Stanford University, USA
    • Stanford Univ
  • Thomas P Devereaux

    • Stanford Univ
    • Stanford University; SLAC National Accelerator Laboratory
    • Stanford University
  • Wei-Sheng Lee

    • SLAC - Natl Accelerator Lab