Filming the metal-insulator transition - from T<sub>c</sub>maps to machine learning pattern recognition

ORAL

Abstract

Over recent years, phase separation has been revealed from the nanometer to micron scales in various transition metal oxides. These maps have offered the possibility to extract and analyze cluster size, critical exponents etc… at snapshot temperatures across the transition. Tracking fine changes in the cluster dynamics at slow temperature sweep has, however, not yet been possible. To do so we have developed a 77K-600K variable temperature autofocus microscope operating in the visible range. Up to 1000 images can be typically measured crossing Tc. We will first review the experimental setup and image analysis developed to complete this study. We will then review key results obtained on Vanadium Dioxide, VO2: critical temperature maps (Tc maps), ΔTc hysteretic maps, memory maps, switching maps, resistor network and pattern recognition of clusters using machine learning.

*S.B., F.S., and E.W.C. acknowledge support from NSF Grant No. DMR-2006192 and the Research Corporation for Science Advancement Cottrell SEED Award. S.B. acknowledges support from a Bilsland Dissertation Fellowship. E.W.C. acknowledges support from a Fulbright Fellowship. P.S. and I.S. acknowledge support from AFOSR Grant No. FA9550-20-1-0242. A.Z., L.A. and M.A-B. acknowledge support by the European innovation and research program Horizon 2020 - Marie Sklodowska-Curie Actions (MSCA) - COFUND, AI4theSciences (PSL, France).

Presenters

  • Melissa Alzate Banguero

    • ESPCI Paris

Authors

  • Melissa Alzate Banguero

    • ESPCI Paris
  • Sayan Basak

    • Purdue University
  • Nicolas Raymond

    • ESPCI PSL-Sorbonne University
    • ESPCI PSL-CNRS-Sorbonne University Paris
  • Forrest Simmons

    • Purdue University
  • Pavel Salev

    • University of California, San Diego
  • Ivan K Schuller

    • University of California, San Diego
    • University of California San Diego
  • Lionel Aigouy

    • ESPCI PSL-Sorbonne University
    • ESPCI PSL-CNRS-Sorbonne University Paris
    • ESPCI PSL-CNRS
  • Alexandre Zimmers

    • ESPCI PSL-Sorbonne University
    • ESPCI PSL-CNRS-Sorbonne University Paris
  • Erica W Carlson

    • Purdue University