Optimization of Nb Superconducting Films for Quantum Devices by H-T Phase Boundary Analysis

ORAL

Abstract

A critical area for the improvement of quantum devices is the materials optimization of superconducting films used in the construction of qubit elements and resonators, where careful considerations of purity and morphology must be made to reduce the effects of TLSs. In materials such as Nb, this involves simultaneously refining both the interfacial properties of the film as well as the superconductivity of the bulk. 

In this talk I discuss our current approach to assessing materials properties of superconducting films through careful transport studies of the superconducting H-T phase boundary. Our method utilizes a resistance feedback technique to continuously map Tc under applied field and allows for a rapid mapping of the phase diagram and extraction of the coherence length ξ0 in the low field G.L. limit, which in certain cases can be a better indicator of film quality than Tc alone. In addition, non-linearity of the low field limit and transition width broadening are readily observed with high fidelity, opening up additional metrics for evaluation. 

Through comparison of Nb films produced under various growth conditions, we demonstrate the value of our approach in providing detailed assessment of the properties of Nb films of various purities and morphologies.  

*This material is based upon work supported by the U.S. Department of Energy, Office of Science, National Quantum Information Science Research Centers, Superconducting Quantum Materials and Systems Center (SQMS) under contract number DE-AC02-07CH11359. Additional support and equiptment provided by DURIP grant W911NF-20-1-0066.

Presenters

  • Kevin M Ryan

    • Northwestern University

Authors

  • Kevin M Ryan

    • Northwestern University
  • Patrick W Krantz

    • Northwestern University
  • Carlos G Torres Castanedo

    • Northwestern University
    • Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, United States
  • Paul M Das

    • Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, United States
    • Northwestern University
  • KVLV Narayanachari

    • Northwestern University
  • Dominic P Goronzy

    • Northwestern University
    • Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, United States
  • Michael J Bedzyk

    • Northwestern University
    • Department of Physics and Astronomy, Department of Materials Science and Engineering, Northwestern University
  • Vinayak P Dravid

    • Northwestern University
    • Department of Materials Science and Engineering, Northwestern University; International Institute of Nanotechnology, Northwestern University; NUANCE Center, Northwestern U.
  • Mark C Hersam

    • Northwestern University
    • Materials Science and Engineering, Northwestern University, Evanston, IL 60208
  • Antony McFadden

    • National Institute of Standards and Technology
  • Corey Rae McRae

    • National Institute of Standards and Technology
  • Mark Field

    • Rigetti Quantum Computing
    • Rigetti Computing
  • Cameron J Kopas

    • Rigetti Quantum Computing
    • Rigetti Computing
  • Jayss Marshall

    • Rigetti Computing
    • Rigetti Quantum Computing
  • Matthew J Reagor

    • Rigetti Quantum Computing
  • Venkat Chandrasekhar

    • Northwestern University