High cooperativity coupling of nuclear spins in a Yb(trensal) molecular qudit to on-chip superconducting resonators

ORAL

Abstract

In this work we study the coupling of Yb3+ nuclear spin states in a Yb(trensal) molecule to superconducting cavities. Experiments have been performed on magnetically diluted single crystals placed onto the inductor of lumped-element LC superconducting resonators with characteristic frequencies spanning the range of nuclear and electronic spin transitions. An external magnetic field is used to tune the spin transitions on resonance with the resonators. Results show strong coupling of cavity photons to electronic spin states and a high-cooperativity coupling in the case of nuclear spins. The nuclear spin-photon coupling is enhanced by the hyperfine interaction with the electronic spin. Attaining the coherent coupling regime is a requisite to perform non-demolition read-out of the electronic and nuclear spin states. This technology enables the implementation of quantum error correction in crystals of molecular spin qudits.

*We acknowlegde financial support from EU (FATMOLS FETOPEN-RIA-2019-01 862893 and SUMO QuantERA 2017), Spanish MCIU/AEI/FEDER (SUMO PCI2018-093116, SUPERMAN-QUTE RTI2018-096075-B-C21, MADE PID2019-105552RB-C44, and PID2019-105), DGA (E09_20R Q-MAD), ONR-Global (DEFROST #N62909-19-1-2053) and the CSIC Research Platform on Quantum Technologies (PTI-001552RB-C41)

Presenters

  • Victor Rollano

    • Spanish National Research Council (CSIC)

Authors

  • Victor Rollano

    • Spanish National Research Council (CSIC)
  • Marcos Rubin-Osanz

    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.
    • Consejo Superior de Investigaciones Cientificas (CSIC) / Universidad de Zaragoza / INMA
    • Spanish National Research Council (CSIC)
  • Marina C de Ory

    • Spanish National Research Council (CSIC) / Spanish National Institute of Aerospace Technology (INTA)
    • Centro de Astrobiología CSIC-INTA, 28850 Torrejón de Ardoz, Spain
    • Spanish National Research Council (CSIC)
  • Daniel Granados

    • IMDEA Nanociencia, Calle Faraday 9, Campus de Cantoblanco, 28049 Madrid, Spain
    • IMDEA Nanoscience
  • Alessandro Chiesa

    • Università di Parma
  • David Zueco

    • Spanish National Research Council (CSIC) / University of Zaragoza
    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.
    • Consejo Superior de Investigaciones Cientificas (CSIC)
    • Consejo Superior de Investigaciones Cientificas (CSIC) / Universidad de Zaragoza / INMA
    • Spanish National Research Council (CSIC)
  • Alicia Gomez

    • Spanish National Research Council (CSIC) / Spanish National Institute of Aerospace Technology (INTA)
    • Centro de Astrobiología CSIC-INTA, 28850 Torrejón de Ardoz, Spain
    • Spanish National Research Council (CSIC)
  • Stergios Piligkos

    • Univ of Copenhagen
    • University of Copenhagen
  • Stefano Carretta

    • University of Parma
    • Università di Parma
  • Fernando M Luis

    • INMA(CSIC-U. Zaragoza)
    • Spanish National Research Council (CSIC) / University of Zaragoza
    • Instituto de Nanociencia y Materiales de Aragón (INMA), CSIC-Universidad de Zaragoza, C/ Pedro Cerbuna 12, 50009 Zaragoza, Spain.
    • Instituto de Nanociencia y Materiales de Aragón (CSIC-Universidad de Zaragoza)
    • Consejo Superior de Investigaciones Cientificas (CSIC) / Universidad de Zaragoza / INMA
    • Spanish National Research Council (CSIC)