Formation of short-range magnetic order and avoided ferromagnetic quantum criticality in pressurized LaCrGe<sub>3</sub>

ORAL

Abstract

LaCrGe3 has emerged as a model system for the study of the avoidance of ferromagnetic (FM) quantum criticality in itinerant magnets [1,2]. In this talk, we will present our results from combining thermodynamic, transport, x-ray and neutron scattering as well as μSR measurements on LaCrGe3 under pressure to identify the various phases in the phase diagram across the avoided FM quantum-critical point. We present thermodynamic evidence (i) for the first-order character of the FM transition at lowest temperatures and (ii) for the formation of new phases at high pressures. From our microscopic data, we infer that short-range FM ordered clusters rather than long-range modulated antiferromagnetism exist in these high-pressure phases. Overall, our results suggest that the phase diagram of LaCrGe3 combines features that are usually associated with avoided criticality in either clean or strongly disordered FM metals.
[1] Taufour et al., PRL 117, 037207 (2016); [2] Kaluarachchi et al., Nat. Commun. 8, 546 (2017).

*This work was carried out at Iowa State University and supported by Ames Laboratory, US DOE, under Contract No. DE-AC02- 07CH11358. Parts of this work were supported by the Gordon and Betty Moore Foundation, the Keck foundation, DOE, NSF and the Swiss NSF.

Presenters

  • Elena Gati

    • Iowa State University/ Ames Laboratory
    • Ames Lab/Iowa State
    • Ames Lab

Authors

  • Elena Gati

    • Iowa State University/ Ames Laboratory
    • Ames Lab/Iowa State
    • Ames Lab
  • John Wilde

    • Physics and Astronomy, Iowa State University/Ames Laboratory
    • Ames Lab/Iowa State
  • Rustem Khasanov

    • Paul Scherrer Institute
    • Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute
  • Li Xiang

    • Ames Lab/Iowa State
    • Ames Laboratory, U.S. Department of Energy, and Department of Physics and Astronomy, Iowa State University
  • Sachith Dissanayake

    • Department of Physics, Duke University
    • Oak Ridge National Lab
    • Duke University
    • Oak Ridge National Laboratory
  • Ritu Gupta

    • Paul Scherrer Institute
    • Laboratory for Muon Spin Spectroscopy, Paul Scherrer Institute
  • Masaaki Matsuda

    • Oak Ridge National Laboratory
    • Oak Ridge National Lab
    • Neutron Scattering Division, Oak Ridge National Laboratory
    • Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
  • Feng Ye

    • Oak Ridge National Laboratory
    • Oak Ridge National Lab
    • Neutron Scattering Division, Oak Ridge National Laboratory
  • Bianca Haberl

    • Oak Ridge National Laboratory
    • Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, TN, USA
    • Neutron Scattering Division, Oak Ridge National Laboratory
    • Oak Ridge National Lab
  • Udhara Kaluarachchi

    • Ames Lab/Iowa State
  • Robert J McQueeney

    • Ames Lab
    • Physics and Astronomy, Iowa State University/Ames Laboratory
    • Department of Physics and Astronomy, Ames Laboratory, Iowa State University
    • Ames Lab/Iowa State
    • Ames Laboratory, U.S. Department of Energy, Ames, Iowa 50011, USA
    • Iowa State University
    • Ames Laboratory and Iowa State University, Ames, IA USA 50011
    • Ames Laboratory/Iowa State University
  • Andreas Kreyssig

    • Physics and Astronomy, Iowa State University/Ames Laboratory
    • Department of Physics and Astronomy, Ames Laboratory, Iowa State University
    • Ames Lab/Iowa State
    • Ames Laboratory, Iowa State University, Dept. of Physics and Astronomy, Ames
    • Ames Laboratory and Iowa State Univeristy
  • Sergey Budko

    • Iowa State University/ Ames Laboratory
    • Ames Laboratory
    • Physics and Astronomy, Iowa State University/Ames Laboratory
    • Ames Laboratory/Iowa State University
    • Ames Lab/Iowa State
    • Ames Laboratory, Ames, IA
    • Iowa State University/AmesLab
    • Department of Physics & Astronomy, Iowa State University/Ames Laboratory
  • Paul C Canfield

    • Iowa State University/ Ames Laboratory
    • Ames Laboratory
    • Ames Laboratory, Iowa State University
    • Iowa State University
    • Ames Lab/Iowa State
    • Ames Laboratory, Ames, IA
    • Iowa State University/AmesLab
    • Department of Physics and Astronomy, Iowa State University/Ames Laboratory
    • Department of Physics & Astronomy, Iowa State University/Ames Laboratory
    • Ames Laboratory, U.S. Department of Energy, and Department of Physics and Astronomy, Iowa State University
    • Ames Laboratory/Iowa State University