Realization of the orbital-selective Mott state at the molecular level in Ba3LaRu2O9

ORAL

Abstract

Molecular magnets based on heavy transition metals have recently attracted significant interest in the quest for novel magnetic properties. For systems with an odd number of valence electrons per molecule, high or low molecular spin states are typically expected in the double exchange or quasi-molecular orbital limits respectively. In this work, we use bulk characterization, muon spin relaxation, neutron diffraction, and inelastic neutron scattering to identify a rare intermediate spin-3/2 per dimer state that cannot be understood in a double exchange or quasi-molecular orbital picture and instead arises from orbital-selective Mott insulating behavior at the molecular level. Our measurements are also indicative of stripe magnetic order below TN = 25 K for these molecular spin-3/2 degrees-of-freedom, which is consistent with expectations for an ideal triangular lattice with significant next nearest neighbor in-plane exchange. Finally, we present neutron diffraction and Raman spectroscopy data under applied pressure that reveal a coincident crystal symmetry lowering and spin state transition from S = 3/2 to S = 1/2 at a modest pressure P ~ 1 GPa, which highlights the delicate balance between competing energy scales in this system.

Presenters

  • Adam Aczel

    • Oak Ridge National Laboratory
    • Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
    • Neutron Scattering Division, Oak Ridge National Laboratory
    • Oak Ridge National Lab

Authors

  • Adam Aczel

    • Oak Ridge National Laboratory
    • Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
    • Neutron Scattering Division, Oak Ridge National Laboratory
    • Oak Ridge National Lab
  • Qiang Chen

    • Dep. Physics and Astronomy, University of Tennessee, Knoxville TN
    • University of Tennessee
    • Department of Physics and Astronomy, University of Tennessee
  • Aime Verrier

    • Universite de Sherbrooke
  • Djamel Ziat

    • Universite de Sherbrooke
  • Amanda J Clune

    • University of Tennessee
  • Redha Rouane

    • Universite de Sherbrooke
  • Xavier Bazier-Matte

    • Universite de Sherbrooke
  • Jie Ma

    • School of Physics and Astronomy, Shanghai Jiao Tong University
    • Shanghai Jiao Tong University
  • Stuart Calder

    • Oak Ridge National Laboratory
    • Oak Ridge National Lab
    • Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
  • Keith Taddei

    • Oak Ridge National Lab
  • Clarina Dela Cruz

    • Oak Ridge National Lab
    • Materials Science and Technology Division, Oak Ridge National Laboratory
  • Alexander Kolesnikov

    • Spallation Neutron Source, Oak Ridge National Laboratory
    • Neutron Scattering Division, Oak Ridge National Lab
    • Oak Ridge National Lab
    • Neutron Scattering Division, Oak Ridge National Laboratory
    • ORNL
    • Oak Ridge National Laboratory
  • Jinguang Cheng

    • Chinese Academy of Sciences
    • Beijing National Laboratory for Condensed Matter Physics, Institute of Physics
  • Z. Liu

    • University of Illinois at Chicago
  • Jeffrey A Quilliam

    • Universite de Sherbrooke
  • Janice Musfeldt

    • University of Tennessee
    • Department of Physics and Astronomy, Rutgers University
    • Department of Chemistry, University of Tennessee
  • Haidong Zhou

    • Dep. Physics and Astronomy, University of Tennessee, Knoxville TN
    • Department of Physics and Astronomy, University of Tennessee, Knoxville
    • University of Tenessee
    • University of Tennessee, Knoxville
    • Physics and Astronomy, University of Tennessee at Knoxville
    • University of Tennessee
    • Department of Physics and Astronomy, University of Tennessee