Locally induced excitonic complexes in a monolayer WSe<sub>2</sub>

ORAL

Abstract

Monolayer transition metal dichalcogenides support various types of excitonic complexes due to the strong vertical confinement and reduced dielectric screening1. Electrostatic gating plays a crucial role to control the excitonic complexes and enables a wide-range of optoelectronic and quantum applications2. However, gating in a nanoscale region and its effect on the excitonic complexes remains an open question. Here, we show that a conductive nanoscale tip induces a local emission peak around 1.67 eV, which is clearly distinguished from the surrounding area in a monolayer WSe2. Electrical and photophysical experiments reveal that the local peak is energy-tunable and different from trionic or biexcitonic emission. Our results open the possibility of confining and controlling excitonic complexes at cryogenic temperature.

1. M. Barbone et al., Nature Communications 9, 3721 (2018)
2. T. Mueller and E. Malic, npj 2D Materials and Applications 2, 29 (2018)

*This work was supported in part by the Army Research Office (ARO) Multidisciplinary University Research Initiative (MURI) program, grant no. W911NF-18-1-0431, and in part by National Science Foundation (NSF) Research Advanced by Interdisciplinary Science and Engineering (RAISE), grant no. CHE-1839155.

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Presenters

  • Hyowon Moon

    • Massachusetts Institute of Technology MIT

Authors

  • Hyowon Moon

    • Massachusetts Institute of Technology MIT

  • Lukas Mennel

    • Massachusetts Institute of Technology MIT

  • Cheng Peng

    • Massachusetts Institute of Technology MIT

  • Chitraleema Chakraborty

    • Massachusetts Institute of Technology MIT
    • Harvard University

  • Takashi Taniguchi

    • National Institute for Materials Science
    • National Institute for Materials Science, Japan
    • National Institure for Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science
    • NIMS
    • National Institute of Materials Science
    • National Institute for Materials Science (NIMS)
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • National Institute for Materials Science,1-1 Namiki
    • National Institute of Material Science
    • National Institute for Materials Science, Tsukuba, Japan
    • International Center for Materials Nanoarchitectonics, NIMS
    • Research Center for Functional Materials, National Institute for Materials Science
    • National Institute of Materials Science, Tsukuba, Japan
    • National Institude for Materials Science
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science, Tsukuba 305-0044, Japan
    • International Center for Materials Nanoarchitectonics, National Institute for Materials
    • NIMS - Japan
    • National Institute for Materials Science ,Japan
    • National Institute for Materials Science, Tsukuba, 305-0044, Ibaraki, Japan
    • National Institute for Material Science
    • National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science Japan
    • 8International Center for Materials Nanoarchitectonics
    • NIMS Tsukuba
    • National Institute for Materials Science: Namiki, Tsukuba, Ibaraki, JP
    • National Institue for Material Science
    • National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan
    • Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Research Center for Functional Materials, National In
    • Research Center for Functional Materials, Japan
    • Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan
    • International Center for Material Nanoarchitectonics, National Institute for Materials Science
    • International Center for Materials Nanoarchitectonics
    • NIMS Suguba
    • NIMS, Tsukuba, Japan
    • National Cheng Kung University
    • National Institute for Materials Science, Namiki 1-1, Tsukuba, 305-0044, Ibaraki, Japan
    • National institute of material science
    • Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan
    • Advanced Materials Laboratory, NIMS
    • National Institute for Materials Science, International Center for Materials Nanoarchitectonics
    • National Institute of Material Science, Japan
    • Tsukuba, National Institute for Materials Science

  • Kenji Watanabe

    • National Institute for Materials Science
    • National Institute for Materials Science, Japan
    • National Institure for Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science
    • NIMS
    • National Institute of Materials Science
    • National Institute for Materials Science (NIMS)
    • Research Center for Functional Materials, National Institute for Materials Science
    • National Institute for Materials Science,1-1 Namiki
    • National Institute of Material Science
    • National Institute for Materials Science, Tsukuba, Japan
    • Research Center for Functional Materials, NIMS
    • National Institute of Materials Science, Tsukuba, Japan
    • National Institude for Materials Science
    • National Institute for Materials Science, Tsukuba, Ibaraki, Japan
    • Research Center for Functional Materials, National Institute for Materials Science, Tsukuba 305-0044, Japan
    • International Center for Materials Nanoarchitectonics, National Institute for Materials
    • NIMS - Japan
    • National Institute for Materials Science ,Japan
    • National Institute for Materials Science, Tsukuba, 305-0044, Ibaraki, Japan
    • National Institute for Material Science
    • National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science Japan
    • NIMS Tsukuba
    • National Institute for Materials Science, Research Center for Functional Materials, Japan
    • Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Materials Science: Namiki, Tsukuba, Ibaraki, JP
    • National Institue for Material Science
    • National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan
    • Materials, NIMS
    • Research Center for Functional Materials, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan, Research Center for Functional Materials, National In
    • Research Center for Functional Materials, Japan
    • International Center for Materials Nanoarchitectonics, National Institute for Materials Science
    • International Center for Materials nanoarchtectonics, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan
    • NIMS Suguba
    • NIMS, Tsukuba, Japan
    • National Institute for Materials Science, Namiki 1-1, Tsukuba, 305-0044, Ibaraki, Japan
    • National institute of material science
    • Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044, Japan
    • Advanced Materials Laboratory, NIMS
    • Research Center for Functional Materials, National Institute for Materials Science, Ibaraki, Japan
    • National Institute for Materials Science, Research Center for Functional Materials
    • National Institute of Material Science, Japan
    • Tsukuba, National Institute for Materials Science

  • Dirk R. Englund

    • Massachusetts Institute of Technology
    • Massachusetts Institute of Technology MIT
    • Department of Electrical Engineering and Computer Science, Massachusetts Institute of Technology