Localized spin-orbit polaron in magnetic Weyl semimetal Co<sub>3</sub>Sn<sub>2</sub>S<sub>2</sub>

ORAL

Abstract

The transition metal based kagome lattice compounds have merged as a novel platform for exploring the physics of geometric frustration, correlation and magnetism, and the topological behaviors of quantum electronic states. The kagome lattice Co3Sn2S2 exhibits the quintessential topological phenomena of a magnetic Weyl semimetal such as chiral anomaly and Fermi-arc surface states. Probing its magnetic properties is crucial for understanding this correlated topological state. Here, using spin-polarized scanning tunneling microscopy/spectroscopy (STM/S) and non-contact atomic force microscopy (nc-AFM) combined with first-principle calculations, we report the discovery of localized spin-orbit polarons (SOPs) with three-fold rotation symmetry nucleated around single S-vacancies in Co3Sn2S2. The SOPs carry a magnetic moment and a large diamagnetic orbital magnetization of a possible topological origin relating to the diamagnetic circulating current around the S-vacancy. Appreciable magneto-elastic coupling of the SOP is detected by nc-AFM and STM. Our findings suggest the SOPs can enhance magnetism and more robust time-reversal-symmetry-breaking topological phenomena. Controlled engineering of the SOPs may pave the way toward practical applications in functional quantum devices.

Presenters

  • Yuqing Xing

    • Chinese Academy of Sciences,Institute of Physics
    • Institute of Physics, Chinese Academy of Sciences
    • Chinese Academy of Sciences, Institute of Physics

Authors

  • Yuqing Xing

    • Chinese Academy of Sciences,Institute of Physics
    • Institute of Physics, Chinese Academy of Sciences
    • Chinese Academy of Sciences, Institute of Physics
  • Shen Jian Lei

    • Chinese Academy of Sciences, Institute of Physics
  • Hui Chen

    • Chinese Academy of Sciences,Institute of Physics
    • Institute of Physics, Chinese Academy of Sciences
    • Chinese Academy of Sciences, Institute of Physics
  • Li Huang

    • Chinese Academy of Sciences, Institute of Physics
  • Yuxiang Gao

    • Chinese Academy of Sciences, Institute of Physics
  • Qi Zheng

    • Chinese Academy of Sciences, Institute of Physics
  • Yu-Yang Zhang

    • Chinese Academy of Sciences,Institute of Physics
    • University of Chinese Academy of Sciences
    • Institute of Physics and University of Chinese Academy of Sciences, Chinese Academy of Sciences, Beijing 100190, China
    • School of physical sciences, Institute of Physics and University of Chinese Academy of Sciences
    • Institute of Physics, Chinese Academy of Sciences
    • Institute of Physics & University of Chinese Academy of Sciences, Chinese Academy of Sciences
  • Geng Li

    • Chinese Academy of Sciences,Institute of Physics
    • Chinese Academy of Sciences, Institute of Physics
    • Institute of Physics, Chinese Academy of Sciences
  • Bin Hu

    • Chinese Academy of Sciences, Institute of Physics
  • Hechang Lei

    • Renmin university of China
    • Renmin University of China
    • Boston College
    • International Center for Quantum Materials, Peking University
  • Wei Ji

    • Renmin University of China
  • Shixuan Du

    • Chinese Academy of Sciences,Institute of Physics
    • Institute of Physics and University of Chinese Academy of Sciences, Chinese Academy of Sciences, Beijing 100190, China
    • School of physical sciences, Institute of Physics and University of Chinese Academy of Sciences
    • Institute of Physics, Chinese Academy of Sciences
    • Chinese Academy of Science
    • Chinese Academy of Sciences, Institute of Physics
    • Institute of Physics & University of Chinese Academy of Sciences, Chinese Academy of Sciences
  • Xiao Lin

    • University of Chinese Academy of Sciences
  • Enke Liu

    • Chinese Academy of Sciences, Institute of Physics
  • Baogen Shen

    • Chinese Academy of Sciences
  • Ziqiang Wang

    • Boston University
    • Physics, Boston College
    • Boston College
    • Department of Physics, Boston College
  • Hongjun Gao

    • Chinese Academy of Sciences,Institute of Physics
    • Institute of Physics, Chinese Academy of Sciences
    • Chinese Academy of Sciences, Institute of Physics