Realization of the kagome spin ice state in frustrated intermetallic HoAgGe

 · Invited

Abstract

Frustration in spin systems can result in the formation of exotic phases of matter. Spin ices are exotic phases of matter characterized by frustrated spins obeying local “ice rules”, in analogy with the electric dipoles in water ice (1). In two dimensions, one can similarly define ice rules for in-plane Ising-like spins arranged on a kagome lattice (2-3). These ice rules require each triangle plaquette to have a single monopole, and can lead to various unique orders and excitations (2-3). Using experimental and theoretical approaches including magnetometry, thermodynamic measurements, neutron scattering and Monte Carlo simulations, we establish HoAgGe as a crystalline (i.e. non-artificial) system that realizes the kagome spin ice state. The system features a variety of partially and fully ordered states and a sequence of field-induced phases at low temperatures, all consistent with the kagome ice rule (4).
References:
(1) C. Castelnovo, R. Moessner, S. L. Sondhi, Nature 451, 42–45 (2008)
(2) A. S. Wills, R. Ballou, C. Lacroix, Phys. Rev. B 66, 144407 (2002)
(3) Chern, G.-W. et al. Phys. Rev. Lett. 106, 207202 (2011)
(4) Zhao, K. et al. Science 367, 1218–1223 (2020)

*The work in Augsburg was supported by the German Science Foundation through SPP1666 (project number 220179758) and TRR80 (project number 107745057). The instrument POLI at Heinz Maier-Leibnitz Zentrum (MLZ), Garching, Germany, was operated by RWTH Aachen University in cooperation with FZ Jülich (Jülich Aachen Research Alliance JARA). The spectrometer NEAT was operated by Helmholtz Zentrum Berlin. This work utilized the RMACC Summit supercomputer, which is supported by the National Science Foundation (awards ACI-1532235 and ACI-1532236), the University of Colorado Boulder, and Colorado State University. The Summit supercomputer is a joint effort of the University of Colorado Boulder and Colorado State University. The work in Prague was supported by the Czech Science Foundation through Project No. 18-10504S.

Presenters

  • Kan Zhao

    • Center for Electronic Correlations and Magnetism, Augsburg University

Authors

  • Kan Zhao

    • Center for Electronic Correlations and Magnetism, Augsburg University