Cluster Aggregation in Bosonic and Fermionic Helium Nanodroplets

ORAL

Abstract

Bosonic superfluid helium-4 droplets obtained in molecular beams have sizable angular momentum, which manifests itself physically in the form of quantized vortices. In our previous works, vortices have been visualized via ultrafast X-ray coherent diffractive imaging using xenon as a contrast agent. Xenon atoms are attracted to the vortex cores leading to the formation of filament – shaped clusters [1]. Here, we study the formation of clusters in non-superfluid fermionic helium-3 droplets, which also rotate but are devoid of any quantum vortices. It was found that in distinction to helium-4, xenon atoms inside helium-3 form loose aggregates arranged into rings on the periphery of the droplets. This is because in normal fluid helium-3 droplets, dopants are fixed in the rotating frame. Thus, heavy xenon atoms are pushed to the droplets’ periphery by centrifugal forces where they recombine into ring-shaped structures.

*This material is based upon work supported by the National Science Foundation under Grant No. DMR-1701077 (A.F.V.). Use of the Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515.

Presenters

  • Alexandra J Feinberg

    • Univ of Southern California

Authors

  • Alexandra J Feinberg

    • Univ of Southern California
  • Deepak Verma

    • Univ of Southern California
  • Sean O'Connell

    • Univ of Southern California
  • Swetha Erukala

    • Univ of Southern California
  • Rico Tanyag

    • Univ of Southern California
  • Weiwu Pang

    • Univ of Southern California
  • Catherine Saladrigas

    • Lawrence Berkeley National Lab
  • Benjamin W Toulson

    • Lawrence Berkeley National Lab
    • Lawrence Berkeley National Laboratory
  • Mario Borgwardt

    • Lawrence Berkeley National Lab
  • Niranjan Shivaram

    • SLAC National Lab
  • Ming-Fu Lin

    • SLAC - Natl Accelerator Lab
    • SLAC National Lab
    • SLAC Natl Accelerator Lab
  • Andre Al Haddad

    • Paul Scherrer Institut
  • Wolfgang Jäeger

    • University of Alberta
  • Christoph Bostedt

    • Paul Scherrer Institut
    • École Polytechnique Fédérale de Lausanne
  • Peter Walter

    • SLAC National Lab
  • Oliver Gessner

    • Lawrence Berkeley National Laboratory
    • Lawrence Berkeley National Lab
  • Andrey F. Vilesov

    • Univ of Southern California