Twenty millisecond electron-spin coherence in an erbium doped crystal

ORAL

Abstract

Rare-earth-ions are interesting physical systems because they have long lived states and record coherence times for both the optical and nuclear transitions [1]. Rare-earths with an odd number of electrons are also paramagnetic, with an electron-spin transition at GHz frequencies in magnetic fields less than 1 Tesla. For such transitions, coherence times up to 2 ms have been measured at temperatures greater than 100mK [2]. Here we present our recent EPR results in 50 ppm and 10 ppb Er doped CaWO4. These measurements were recorded in a previously unstudied temperature regime for this material: sub-Kelvin temperature down to 10mK, using a superconducting micro-resonator and a superconducting parametric amplifier [3]. We observe the longest recorded Hahn-echo decay for an electronic spin transition in an Erbium doped material, up to 20 ms.
[1] Zhong, M. et al., Nature 517, 177-180 (2015).
[2] Li, P. et al., Phys. Rev. Appl 13, 024080 (2020)
[3] A. Bienfait et al., Nature nanotechnology, vol. 11, no 3, p. 253, (2016)

*We acknowledge Lincoln Labs for providing a Parametric Amplifier. We thank the Chaire Industrielle NASNIQ (grant ANR-17-CHIN-0001) supported by Atos, the project QIPSE (grant ACUHK403/15), the project MIRESPIN, SIRTEQ grant REIMIC and EU grant SMERC (792727).

Presenters

  • Marianne Le Dantec

    • Quantronics Group, SPEC, CEA Saclay, Saclay, France

Authors

  • Marianne Le Dantec

    • Quantronics Group, SPEC, CEA Saclay, Saclay, France
  • Milos Rancic

    • Quantronics Group, SPEC, CEA Saclay, Saclay, France
  • Emmanuel Flurin

    • CEA-Saclay
    • Quantronics Group, SPEC, CEA Saclay, Saclay, France
  • Denis Vion

    • CEA-Saclay
    • Quantronics Group, SPEC, CEA Saclay, Saclay, France
  • Daniel Esteve

    • CEA-Saclay
    • Quantronics Group, SPEC, CEA Saclay, Saclay, France
  • Patrice Bertet

    • CEA-Saclay
    • Quantronics Group, SPEC, CEA Saclay, Saclay, France
  • Philippe Goldner

    • Chimie ParisTech, PSL University, Paris, France
  • Thierry Chanelière

    • Institut Néel, Univ. Grenoble Alpes, Grenoble, France
  • Bertaina Sylvain

    • Inst. Mat. Microelectronique et Nanosciences de Provence, Aix-Marseille Universite, Marseille, France
    • Inst Mat Microelectronique et Nanosciences de Provence, UMR7334, CNRS, Aix- Marseille Universite, Marseille, France
    • IM2NP, Faculté des Sciences et Techniques, Marseille, France
  • Sen Lin

    • Department of Physics and The Hong Kong Institute of Quantum Information Science and Technology, The Chinese University of Hong Kong, Hong Kong, China
  • Ren Bao Liu

    • Department of Physics and The Hong Kong Institute of Quantum Information Science and Technology, The Chinese University of Hong Kong, Hong Kong, China