High-order fractal quantum oscillations in highly doped graphene/BN superlattices

ORAL

Abstract

High temperature quantum oscillations have been reported in graphene/BN superlattices beyond secondary Dirac points both for electron and hole doping [1,2]. These so-called Brown-Zak (BZ) oscillations originate from periodic emergence of delocalized Bloch states in high magnetic field. However, the BZ oscillations is much less visible for hole doping than for electron doping due to strong electron-hole asymmetry. Here, we employed a newly developed electron beam doping technique to induce high electron and hole carrier densities in graphene/BN superlattices while maintaining high mobilities. Enhanced BZ oscillations are observed beyond the third-generation neutrality points at high temperatures. High-order magnetic Bloch states are also seen even for hole doping, demonstrating the effectiveness of our doping technique. Theoretical simulation of the magnetotransport provides qualitative agreement of the carrier density dependence of BZ oscillations with our experimental results.

References:
[1] R. K. Kumar, X. Chen, et al, Science 357, 181 (2017).
[2] R. K. Kumar, A. Mishchenko, et al, PNAS 115, 5135 (2018).

*This work was supported in part by the U.S. Department of Energy under Contract No. DE-AC02-05-CH11231, within the sp2-Bonded Materials Program (KC2207).

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Presenters

  • Wu Shi

    • Lawrence Berkeley National Lab and UC Berkeley

Authors

  • Wu Shi

    • Lawrence Berkeley National Lab and UC Berkeley

  • Salman Kahn

    • Lawrence Berkeley National Lab and UC Berkeley

  • Takashi Taniguchi

    • National Institute for Materials Science, Japan
    • National Institute for Material Science
    • National Institute for Materials Science
    • National Institute for Materials Science, Tsukuba
    • Research Center for Functional Materials, NIMS
    • nims
    • Advanced Materials Laboratory, National Institute for Materials Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • NIMS
    • National Institute for Material Science - Japan
    • NIMS Tsukuba
    • National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan.
    • National Institute for Materials Science (NIMS)
    • National Institute for Materials Science,Tsukuba, Ibaraki 305-0047, Japan
    • Advanced Materials Laboratory, NIMS, Japan
    • National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan
    • National Institute of Materials Science
    • National Institute for Materials Science, University of Tsukuba
    • National Institute for Materials Science, Tsukuba, Japan
    • National Institue for Material Science, Tsukuba
    • Advanced Materials Laboratory, NIMS
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba 305-0044, Japan
    • Advanced Matrials Lab, NIMS
    • National Institute for Material Science, Tsukuba, Japan
    • National institute for materials science
    • NIMS-Tsukuba
    • NIMS, Japan
    • National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan
    • NIMS Japan
    • National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki, Japan
    • Advanced Materials Laboratory, National Institute of Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science 1-1 Namiki, Tsukuba, 305-0044, Japan
    • National Institute of Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science (Japan)
    • Physics, NIMS
    • National Institute of Materials Science, Japan
    • National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • NIMS - Tsukuba

  • Kenji Watanabe

    • National Institute for Materials Science, Japan
    • National Institute for Material Science
    • National Institute for Materials Science
    • National Institute for Materials Science, Tsukuba
    • Research Center for Functional Materials, NIMS
    • nims
    • Advanced Materials Laboratory, National Institute for Materials Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • NIMS
    • National Institute for Material Science - Japan
    • NIMS Tsukuba
    • National Institute for Materials Science, Namiki 1-1, Ibaraki 305-0044, Japan.
    • National Institute for Materials Science (NIMS)
    • National Institute for Materials Science,Tsukuba, Ibaraki 305-0047, Japan
    • Advanced Materials Laboratory, NIMS, Japan
    • National Institute for Materials Science,1-1 Namiki, Tsukuba, 305-0044, Japan
    • National Institute of Materials Science
    • National Institute for Materials Science, University of Tsukuba
    • National Institute for Materials Science, Tsukuba, Japan
    • National Institute for Material Science, Japan
    • National Institue for Material Science, Tsukuba
    • Advanced Materials Laboratory, NIMS
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba 305-0044, Japan
    • Advanced Matrials Lab, NIMS
    • National Institute for Material Science, Tsukuba, Japan
    • National institute for materials science
    • NIMS-Tsukuba
    • NIMS, Japan
    • National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan
    • NIRM
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan
    • NIMS Japan
    • National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • Research Center for Functional Materials, National Institute for Materials Science, Tsukuba, Ibaraki, Japan
    • Advanced Materials Laboratory, National Institute of Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science 1-1 Namiki, Tsukuba, 305-0044, Japan
    • National Institute of Material Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science (Japan)
    • Physics, NIMS
    • National Institute of Materials Science, Japan
    • National Institute of Materials Science (NIMS)
    • National Institute of Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • NIMS - Tsukuba

  • Michael F Crommie

    • Lawrence Berkeley National Lab and UC Berkeley
    • University of California, Berkeley

  • Alex Zettl

    • Lawrence Berkeley National Lab and UC Berkeley
    • University of California, Berkeley
    • Department of Physics, University of California, Berkeley