Magnetic textures in single crystals of Ni<sub>1-x</sub>Fe<sub>x</sub>Br<sub>2</sub>

ORAL

Abstract

Recently, frustrated systems with finite easy axis anisotropy have been proposed as a route to realize topological spin textures. In this context, Ni1-xFexBr2 has been predicted to host a field-induced skyrmion phase. This presentation will discuss the magnetic properties of Ni1-xFexBr2 single crystals and the magnetic field-temperature phase diagram. NiBr2 crystallizes in the centrosymmetric CdCl2 structure type. It exhibits a commensurate antiferromagnetic phase below TN = 48 K and an incommensurate helimagnetic phase below TIC = 22 K, both with easy plane anisotropy. The helimagnetic structure of Ni1-xFexBr2 is tuned as a function of composition and applied magnetic field, as demonstrated using bulk measurements and neutron scattering. A change in magnetic anisotropy from easy plane to easy axis is observed around x = 0.07, which is expected as a key feature to realize a skyrmion phase in this system.

*U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division

Presenters

  • Binod Rai

    • Materials Science and Technology Division, Oak Ridge National Laboratory
    • Oak Ridge National Laboratory

Authors

  • Binod Rai

    • Materials Science and Technology Division, Oak Ridge National Laboratory
    • Oak Ridge National Laboratory
  • Hasitha Suriya Arachchige

    • Physics and Astronomy, The University of Tennessee
    • Department of Physics & Astronomy, University of Tennessee, Knoxville
    • Department of Physics, University of Tennessee
    • University of Tennessee
    • Department of Physics and Astronomy, The University of Tennessee
  • Ganesh Pokharel

    • Physics, University of Tennessee
    • Physics and Astronomy, The University of Tennessee
    • Department of Physics & Astronomy, University of Tennessee, Knoxville
    • University of Tennessee
    • Department of Physics and Astronomy, The University of Tennessee
    • University of Tennessee, Knoxville
  • Yaohua Liu

    • Neutron Scattering Division, Oak Ridge National Laboratory
    • Oak Ridge National Lab
    • Oak Ridge National Laboratory
  • Shizeng Lin

    • Theoretical Division, Los Alamos National Laboratory
    • Los Alamos Natl Lab
    • Theoretical Division, T-4, Los Alamos National Laboratory
    • Los Alamos National Laboratory
    • Theoretical Division, Los Alamos National Lab
    • Theoretical Division, T-4 and CNLS, Los Alamos National Laboratory
    • Los Alamos National Lab
  • Cristian Batista

    • Physics and Astronomy, The University of Tennessee
    • Neutron Scattering Division and Shull-Wollan Center, Oak Ridge National Laboratory
    • Department of Physics and Astronomy, The University of Tennessee
    • University of Tennessee, Knoxville
    • Department of Physics and Astronomy, University of Tennessee, Knoxville
    • Department of Physics and Astronomy, University of Tennessee
  • David Mandrus

    • Physics, University of Tennessee
    • Materials Science and Engineering, The University of Tennessee
    • Department of Materials Science & Engineering, University of Tennessee, Knoxville
    • The University of Tennesse, Knoxville
    • University of Tennessee
    • Department of Physics and Astronomy, University of Tennessee
    • Oak Ridge National Laboratory
    • Department of Materials Science and Engineering, University of Tennessee Knoxville
    • Department of Materials Science and Engineering, University of Tennessee
    • University of Tennessee, Knoxville
    • Material Science and Technology Division, Oak Ridge National Laboratory
    • Material Science and Technology Division, Oak Ridge National Lab
  • Andrew D Christianson

    • Materials Science & Technology Division, Oak Ridge National Laboratory
    • Materials Science and Technology Division, Oak Ridge National Laboratory
    • Oak Ridge National Lab
    • Materials Science and Technology Division, Oak Ridge National Lab
    • Materials Science and Technology Division, OakRidge National Laboratory
  • Andrew May

    • Materials Science and Technology Division, Oak Ridge National Laboratory
    • Materials Science & Technology Division, Oak Ridge National Laboratory
    • Oak Ridge National Laboratory
    • Oak Ridge National Lab