Time-resolved ARPES signatures of pump driven normal-to-excitonic insulator transition

ORAL

Abstract

We consider a ground-state band insulator turning into a nonequilibrium excitonic insulator (EI) when pumping it at sub-gap frequencies slighlty larger than the excitonic energy. The macroscopic polarization in the non-equilibrium EI phase is characterized by self-sustained oscillations with a frequency depending on the absorbed energy. We show that during the pump-driving the excitonic ARPES structure undergoes a convex-to-concave shape transition and concomitantly the system goes through a BEC-BCS crossover. Furthermore attosecond pulses shone after the pump-driving at different times tdelay generate a photocurrent which oscillates in tdelay. This phenomenon is related to the AC response of an exotic Josephson junction.

*1) RISE Co-ExAN (Grant No. GA644076)
2) European Union project MaX Materials design at the eXascale H2020-EINFRA-2015-1, Grant Agreement No. 676598
3) Nanoscience Foundries and Fine Analysis-Europe H2020-INFRAIA-2014-2015, Grant Agreement No. 654360
4) MIUR PRIN Grant No. 20173B72NB


Presenters

  • Enrico Perfetto

    • Physics Department, Univ of Roma

Authors

  • Enrico Perfetto

    • Physics Department, Univ of Roma
  • Davide Sangalli

    • ISM, CNR
    • FLASHit, CNR-ISM
    • Istituto di Struttra della materia (ISM), CNR
  • Andrea Marini

    • ISM, CNR
  • Gianluca Stefanucci

    • Physics Department, Univ of Roma
    • Physics, University of Rome Tor Vergata