Chemical control of magnetism in <i>S</i> = 1 quantum materials: new twists on a seemingly old theme

 · Invited

Abstract

We aim to control the spatial exchange and single-ion anisotropies (D) in bespoke S = 1 Ni(II) quantum magnets. Early work led to [Ni(HF2)(pyz)2]SbF6 (pyz = pyrazine) which contains Ni-FHF-Ni chains (JFHF) cross-linked by Ni-pyz-Ni segments (Jpyz) to form a tetragonal network [1]. The material undergoes XY-AFM order below TN = 12.2 K with collinear Ni(II) moments confined to the [Ni(pyz)2]2+ plane. High-field M(H) and inelastic neutron scattering (INS) revealed DJFHF >> Jpyz. In the related square lattices [2,3], NiX2(pyz)2 (X = F, Cl, Br, I, NCS), the electronegativity of X dictates the Ni(II) spin direction with XY- and Ising-like ground-states observed for X = F, Cl and X = Br, I, NCS, respectively. We used INS to determine Jpyz and J. Chemical substitution of pyz for pyrimidine (pym) affords unusual topologies and enhanced magnetic interactions along Ni-pym-Ni relative to Ni-pyz-Ni. Thus, we synthesized two new Q1D chains: staggered [Ni(pym)(H2O)4]SO4●2H2O and chiral [Ni(pym)(H2O)4]SiF6●H2O, each showing multiple field-induced phase transitions below 5 K. Lastly, we will describe a unique 3D chiral Ni(II) framework that may display spin-liquid behavior at low temperatures. Time permitting, the structural and magnetic properties of these materials will be discussed.

*NSF DMR-1703003 (EWU), DMR-1157490 (MagLab), DoE, State of FL, ERC, EPSRC

References:
[1] J. Brambleby, et al. Phys. Rev. B (2017) 95, 134435.
[2] J. Liu, et al. Inorg. Chem. (2016) 55, 3515.
[3] J. L. Manson, et al. Polyhed. (2019) submitted and unpublished work.

Presenters

  • Jamie Manson

    • Department of Chemistry and Biochemistry, Eastern Washington University
    • Eastern Washington University

Authors

  • Jamie Manson

    • Department of Chemistry and Biochemistry, Eastern Washington University
    • Eastern Washington University
  • Jacqueline Villa

    • Department of Chemistry and Biochemistry, Eastern Washington University
    • Eastern Washington University
  • Danielle Y. Villa

    • Eastern Washington University
  • Isabel Calderon-Lin

    • Eastern Washington University
  • Zachary Manson

    • Eastern Washington University
  • Nathan Grinalds

    • Eastern Washington University
  • Ashley Sargent

    • Eastern Washington University
  • William Blackmore

    • Physics, University of Warwick
  • Sam Curley

    • Department of Physics, University of Warwick
    • Univ of Warwick
    • Physics, University of Warwick
  • Paul Goddard

    • Physics, Warwick University
    • Department of Physics, University of Warwick
    • Univ of Warwick
    • Physics, University of Warwick
    • University of Warwick
  • John Singleton

    • National High Magnetic Field Lab, Los Alamos
    • Los Alamos National Laboratory
    • NHMFL, Los Alamos National Laboratory
    • National High Magnetic Field Laboratory, Los Alamos National Laboratory
    • NHMFL, Los Alamos National Lab
    • Los Alamos National Lab.
  • Matthew Stone

    • Oak Ridge National Lab
    • Neutron Scattering Division, Oak Ridge National Laboratory
    • Quantum Condensed Matter Div, Oak Ridge National Lab
    • Oak Ridge National Laboratory
    • Spallation Neutron Source, Oak Ridge National Laboratory
    • Neutron Scattering Division, Oak Ridge National Lab
    • Neutron Scattering Division, OakRidge National Laboratory
  • Roger Johnson

    • Physics, University of Oxford
  • Vasile O Garlea

    • Oak Ridge National Laboratory
    • Quantum Condensed Matter Div, Oak Ridge National Lab
    • Oak Ridge National Lab
    • Oak Ridge National Lab, Neutron Scattering Division
  • Pascal Manuel

    • ISIS Facility, Rutherford Appleton Laboratory-STFC
    • ISIS Neutron Source
    • ISIS, STFC RAL
    • ISIS facility, Rutherford Appleton Laboratory
    • ISIS, Rutherford Appleton Laboratory
    • ISIS, Rutherford Appleton Laboratory, UK
  • Craig Brown

    • Center of Neutron Research, National Institute of Standards and Technology
    • NIST Center for Neutron Research
    • NIST Center for Neutron Research, NIST
    • Center for Neutron Research, National Institute of Standards and Technology
    • National Institute of Standards and Technology
    • NCNR, NIST