Cavity nano-optics with configurable interaction: room temperature strong coupling of single emitter

ORAL

Abstract

Quantum state control of two-level emitters is fundamental for many information processing, metrology, and sensing applications. However, quantum-coherent photonic control of solid-state emitters has traditionally been limited to cryogenic environments, which are not compatible with implementation in scalable, broadly distributed technologies. In contrast, plasmonic nano-cavities with deep sub-wavelength mode volumes have recently emerged as a path towards room temperature quantum state hybridization and control. Here we establish plasmonic tip-enhanced strong coupling (TESC) with a configurable nano-tip cavity to modulate and control the cavity-emitter interaction with sub-nanometer precision, quantify coupling strength exceeding ~160 meV, at mode volumes of < 10-6 λ3, augmented by theoretical modeling. Based on this work, we provide a perspective for nano-cavity optics as a promising tool for room temperature control of quantum coherent interactions that could spark new innovations in fields from quantum information and quantum sensing to quantum chemistry and molecular opto-mechanics.

Presenters

  • Markus B. Raschke

    • University of Colorado, Boulder
    • Physics and Chemistry, University of Colorado, Boulder
    • University of Colorado Boulder
    • Department of Physics, Department of Chemistry, and JILA, University of Colorado - Boulder
    • Department of Physics, Department of Chemistry and JILA, University of Colorado, Boulder
    • Department of Physics, Department of Chemistry, and JILA, University of Colorado, Boulder
    • Physics, University of Colorado, Boulder
    • Physics, Chemistry, and JILA, University of Colorado, Boulder

Authors

  • Molly A. May

    • University of Colorado, Boulder
    • Department of Physics, Department of Chemistry, and JILA, University of Colorado - Boulder
  • David Fialkow

    • University of Maryland, Baltimore County
  • Tong Wu

    • Institute d'Optique, CRNS, University of Bordeaux
  • Kyoung-Duck Park

    • University of Colorado, Boulder
    • Department of Physics, Department of Chemistry, and JILA, University of Colorado, Boulder
    • Physics, Chemistry, and JILA, University of Colorado, Boulder
  • Haixu Leng

    • University of Maryland, Baltimore County
  • Jaron Kropp

    • Univ of Maryland-Baltimore County
    • University of Maryland, Baltimore County
  • Theodosia Gougousi

    • Univ of Maryland-Baltimore County
    • University of Maryland, Baltimore County
  • Philippe Lalanne

    • Institute d'Optique, CRNS, University of Bordeaux
  • Matthew A Pelton

    • University of Maryland, Baltimore County
  • Markus B. Raschke

    • University of Colorado, Boulder
    • Physics and Chemistry, University of Colorado, Boulder
    • University of Colorado Boulder
    • Department of Physics, Department of Chemistry, and JILA, University of Colorado - Boulder
    • Department of Physics, Department of Chemistry and JILA, University of Colorado, Boulder
    • Department of Physics, Department of Chemistry, and JILA, University of Colorado, Boulder
    • Physics, University of Colorado, Boulder
    • Physics, Chemistry, and JILA, University of Colorado, Boulder