Enhanced Zeeman splitting in MoS<sub>2 </sub>monolayers doped with transition metals.

ORAL

Abstract

We developed an approach to dope MoS2 monolayers with controllable concentration of transition metal ions. In this approach, a single phase transition metal-doped MoO3 compound precursor was utilized to deposit ultrathin doped MoO3 film by electron beam evaporation, followed by sulfurization of the precursor oxide layer to achieve monolayer transition metal doped MoS2.
We have used magneto-reflectance spectroscopy to compare the Zeeman splitting of MoS2 monolayers with that of MoS2 doped with transition metals. At T = 7K we find that the A-exciton Zeeman splitting in the doped sample is 23% higher that of the undoped MoS2. The enhancement is attributed to exchange interaction between the spins of carriers and those of the transition metal ions.

Presenters

  • Arinjoy Bhattacharya

    • Department of Physics, State University of New York at Buffalo, Buffalo, New York
    • Physics, State Univ of NY - Buffalo, Buffalo, New York

Authors

  • Arinjoy Bhattacharya

    • Department of Physics, State University of New York at Buffalo, Buffalo, New York
    • Physics, State Univ of NY - Buffalo, Buffalo, New York
  • Mengying Bian

    • State Univ of NY - Buffalo
    • Physics, State Univ of NY - Buffalo, Buffalo, New York
  • Arman Najafi

    • Department of Physics, State University of New York at Buffalo, Buffalo, New York
    • Physics, State Univ of NY - Buffalo, Buffalo, New York
  • Peijian Wang

    • State Univ of NY - Buffalo
    • Physics, University at Buffalo
    • Physics, State Univ of NY - Buffalo, Buffalo, New York
  • Alireza Jalouli

    • State Univ of NY - Buffalo
    • Physics, State Univ of NY - Buffalo, Buffalo, New York
  • Jieqiong Wang

    • MOE Key Laboratory of Nonequilibrium Synthesis and Modulation of Condensed Matter, Xi'an Jiaotong University, China
  • Jiadong Zhou

    • Materials Science and Engineering, Nanyang Technological University, Singapore
  • Sen Yang

    • MOE Key Laboratory of Nonequilibrium Synthesis and Modulation of Condensed Matter, Xi'an Jiaotong University, China
  • Zheng Liu

    • Materials Science and Engineering, Nanyang Technological University, Singapore
  • Hao Zeng

    • State Univ of NY - Buffalo
    • Physics, State Univ of NY - Buffalo
    • Physics, University at Buffalo
    • Physics, State Univ of NY - Buffalo, Buffalo, New York
    • State University of New York at Buffalo
  • Athos Petrou

    • Department of Physics, State University of New York at Buffalo, Buffalo, New York
    • Physics, State Univ of NY - Buffalo, Buffalo, New York