Self-assembly of DNA origami particles into self-limited surfaces

ORAL

Abstract

The combination of proteins’ unique folded shapes and specific interactions enable them to self-assemble into functional, nanostructured materials, such as viral capsids and microtubules. In this talk, I will present experimental results showing that we can mimic these features using DNA origami. We devise a scheme for designing synthetic building blocks with prescribed shapes and specific interactions. Our building blocks are DNA origami triangles, which bind via DNA base stacking interactions between shape-complementary edges. The dihedral angles between neighboring building blocks can be tuned independently by designing the building-block geometry. We illustrate our design approach by making triangular building blocks that assemble into self-limited structures, like a zigzag nanotube which is limited in size along one dimension. Molecular dynamics simulations, gel electrophoresis, and electron microscopy verify the three-dimensional structures of the individual building blocks as well as their assemblies. Going forward, our design method will enable us to create other building blocks that self-assemble into surfaces with user-prescribed curvatures.

*We acknowledge financial support from NSF MRSEC DMR-1420382.

Presenters

  • Daichi Hayakawa

    • Physics, Brandeis University

Authors

  • Daichi Hayakawa

    • Physics, Brandeis University
  • Douglas Hall

    • University of Massachusetts Amherst
    • Univ of Mass - Amherst
    • Polymer Science and Engineering, University of Massachusetts Amherst
  • Chris SIgl

    • Physics, Technische Universität München
    • Physics, TUM
  • Gregory Grason

    • Univ of Mass - Amherst
    • Polymer Science, University of Massachusetts
    • University of Massachusetts - Amherst
    • University of Massachusetts Amherst
    • UMass Amherst
    • Polymer Science and Engineering, University of Massachusetts Amherst
  • William Rogers

    • Physics, Brandeis University
    • Brandeis Univ