Disentangled transitions in artificial rare-earth nickelates

ORAL

Abstract

The observation of simultaneous metal-insulator transition, charge ordering transition, and structural transition in rare-earth nickelates hinders our understanding of the underlying mechanism. We have devised a series of new superlattices by combining EuNiO3 and LaNiO3 to form ultrashort period superlattices, which allow one to disentangle the simultaneous orderings. Tailoring an incommensurate heterostructure period relative to the bulk charge ordering pattern suppresses the charge order transition while preserving metal-insulator and antiferromagnetic transitions. Such selective decoupling of the entangled phases resolves the long-standing puzzle about the driving force behind the metal-insulator transition and points to the site-selective Mott transition as the operative mechanism.

Presenters

  • Srimanta Middey

    • Department of Physics, Indian Institute of Science
    • Indian Institute of Science

Authors

  • Srimanta Middey

    • Department of Physics, Indian Institute of Science
    • Indian Institute of Science
  • Derek Meyers

    • University of California, Berkeley
    • Brookhaven National Laboratory
    • Oklahoma State University
  • Mikhail Kareev

    • Physics and Astronomy, Rutgers University
    • Rutgers University, New Brunswick
    • Rutgers University
  • Yanwei Cao

    • Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences
    • Rutgers University
  • Xiaoran Liu

    • Physics and Astronomy, Rutgers University
    • Rutgers University, New Brunswick
    • Rutgers University
  • Padraic Shafer

    • Lawrence Berkeley National Lab
    • Advanced Light Source, LBNL
    • Advanced Light Source
    • Lawrence Berkeley National Laboratory, Advanced Light Source
    • Advanced Light Source, Lawrence Berkeley National Laboratory
    • Lawrence Berkeley National Laboratory
  • John William Freeland

    • Advanced Photon Source, Argonne National Lab
    • Argonne National Lab
    • Advanced Photon Source, Argonne National Laboratory, Argonne, IL, USA
    • Argonne National Laboratory
    • Advanced Photon Source, Argonne National Laboratory
  • J.-W. Kim

    • Advanced Photon Source
    • Argonne National Laboratory
  • P. J. Ryan

    • Argonne National Lab
    • Argonne National Laboratory
  • Jak Chakhalian

    • Physics and Astronomy, Rutgers University
    • Rutgers University, New Brunswick
    • Rutgers University