The role of Joule heating in the voltage-triggered insulator-to-metal transition in VO<sub>2</sub>.

ORAL

Abstract

VO2 undergoes a conductivity increase of up to five orders of magnitude as the temperature is increased through 341 K. Recently, the insulator-to-metal transition (IMT) has been triggered with an applied voltage, but debate remains as to whether the transition can be due to electric field effects alone, or whether Joule heating is necessary. Here, we use a conductive AFM tip to locally apply a voltage bias and measure the current through a VO2 film. By fitting the IV curves immediately preceding the IMT to the temperature-dependent Poole-Frenkel conduction mechanism, we determine the local temperature of VO2 in the insulating state. We find that the tip has locally warmed the film to 335 K ± 4 K immediately preceding the transition. Therefore, Joule heating plays a significant role in the voltage-triggered IMT in VO2.

*AS was funded by NSERC CGSM #6563, JDH was funded by Gordon and Betty Moore Foundation EPiQS Initiative Grant No. GBMF4536, NSF Grant No. DMR-1231319, sample fabrication funded by AFOSR Grant No. FA9550- 08-1-0203.

Presenters

  • Alyson Spitzig

    • Physics, Harvard University

Authors

  • Alyson Spitzig

    • Physics, Harvard University
  • Alex J Frenzel

    • Physics, Harvard University
  • Jeehoon Kim

    • Physics, Harvard University
  • Changhyun Ko

    • SEAS, Harvard University
  • Shriram Ramanathan

    • School of Materials Engineering, Purdue University
    • Purdue University - USA
  • Jennifer Hoffman

    • Physics, Harvard University
    • Department of Physics, Harvard University
    • Harvard University
    • Department of Physics, Harvard University, Cambridge, MA, United States
  • Jason D Hoffman

    • Physics, Harvard University