Structural and electronic properties of doped NiO from density functional theory and quantum Monte Carlo simulations

ORAL

Abstract

NiO is a prototypical strongly correlated oxide. According to band filling, it should be a metal, but correlations drive the ground state to an antiferromagnetic insulator. The general question of how doping affects the electronic – and chemical – structure of correlated oxides is of great fundamental interest, but also important for the realization of electronics,”Mottronics”, based on correlated materials. We are studying hole- and electron-doped NiO using density functional theory (DFT) methods and much more accurate quantum Monte Carlo simulations and compare our results directly with experimental results on high-quality thin films grown by molecular beam epitaxy. One surprising result is that DFT in all flavors we have used fails to properly account for the K-O bond distance, and underestimates it by over 0.3 A compared to analysis based on extended X-ray absorption fine structure. Preliminary results using QMC show much better agreement with experiments, indicating that correlation effects beyond DFT have a dramatic effect on the energy landscape around the dopant.

*Supported by the U.S. DOE, Office of Science, BES, Materials Sciences and Engineering Division, as part of the Comp. Materials Sciences Program and Center for Predictive Simulation of Functional Materials.

Presenters

  • Olle Heinonen

    • Argonne National Laboratory
    • Materials Science Division, Argonne National Laboratory
    • Materials Science Division, Argonne National Laboratory, Lemont, Illinois, USA

Authors

  • Olle Heinonen

    • Argonne National Laboratory
    • Materials Science Division, Argonne National Laboratory
    • Materials Science Division, Argonne National Laboratory, Lemont, Illinois, USA
  • Hyeondeok Shin

    • Argonne National Laboratory
  • Jaron Krogel

    • Oak Ridge National Laboratory
    • Materials Science and Technology Division, Oak Ridge National Laboratory
  • Panchapakesan Ganesh

    • Center for Nanophase Materials Sciences, Oak Ridge National Laboratory
    • Oak Ridge National Lab
    • Oak Ridge National Laboratory
    • Center for Nanophase Materials and Sciences, Oak Ridge National Laboratory
  • Friederike Wrobel

    • Argonne National Laboratory
  • Anand Bhattacharya

    • Argonne National Laboratory
    • Materials Science Division, Argonne National Laboratory
  • Paul Kent

    • Oak Ridge National Laboratory
    • Center for Nanophase Materials Sciences, Oak Ridge National Laboratory
    • Center for Nanophase Materials and Sciences, Oak Ridge National Laboratory